Identification of the sources of primary organic aerosols at urban schools: A molecular marker approach

被引:3
|
作者
Crilley, Leigh R. [1 ]
Qadir, Raeed M. [2 ,3 ]
Ayoko, Godwin A. [1 ]
Schnelle-Kreis, Juergen [2 ]
Abbaszade, Guelcin [2 ]
Orasche, Juergen [2 ]
Zimmermann, Ralf [2 ,3 ]
Morawska, Lidia [1 ]
机构
[1] Queensland Univ Technol, Inst Hlth & Biomed Innovat, Int Lab Air Qual & Hlth, Brisbane, Qld 4001, Australia
[2] Helmholtz Zentrum Munchen, Joint Mass Spectrometry Ctr Comprehens Mol Analyt, D-85764 Neuherberg, Germany
[3] Univ Rostock, Inst Chem, D-18051 Rostock, Germany
基金
澳大利亚研究理事会;
关键词
Positive matrix factorization; Sources; Primary organic aerosols; Exposure; Schools; POSITIVE MATRIX FACTORIZATION; PARTICULATE AIR-POLLUTION; SOURCE APPORTIONMENT; TRACERS; MATTER; QUANTIFICATION; COMBUSTION; NONPOLAR; COOKING; CARBON;
D O I
10.1016/j.envpol.2014.04.023
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Children are particularly susceptible to air pollution and schools are examples of urban microenvironments that can account for a large portion of children's exposure to airborne particles. Thus this paper aimed to determine the sources of primary airborne particles that children are exposed to at school by analyzing selected organic molecular markers at 11 urban schools in Brisbane, Australia. Positive matrix factorization analysis identified four sources at the schools: vehicle emissions, biomass burning, meat cooking and plant wax emissions accounting for 45%, 29%, 16% and 7%, of the organic carbon respectively. Biomass burning peaked in winter due to prescribed burning of bushland around Brisbane. Overall, the results indicated that both local (traffic) and regional (biomass burning) sources of primary organic aerosols influence the levels of ambient particles that children are exposed at the schools. These results have implications for potential control strategies for mitigating exposure at schools. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:158 / 165
页数:8
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