The ADOR mechanism for the synthesis of new zeolites

被引：279

作者：

Eliasova, Pavla ^{[1
]}

Opanasenko, Maksym ^{[1
]}

Wheatley, Paul S. ^{[2
]}

Shamzhy, Mariya ^{[1
]}

Mazur, Michal ^{[1
]}

Nachtigall, Petr ^{[3
]}

Roth, Wieslaw J. ^{[1
,4
]}

Morris, Russell E. ^{[2
]}

Cejka, Jiri ^{[1
]}

机构：

[1] Acad Sci Czech Republ, J Heyrovsky Inst Phys Chem, Vvi, CR-18223 Prague 8, Czech Republic

[2] Univ St Andrews, EaStChem Sch Chem, St Andrews KY16 9ST, Fife, Scotland

[3] Charles Univ Prague, Fac Sci, Dept Phys & Macromol Chem, Prague 12840 2, Czech Republic

[4] Jagiellonian Univ, Fac Chem, PL-30060 Krakow, Poland

来源：

CHEMICAL SOCIETY REVIEWS | 2015年 / 44卷 / 20期

基金：

英国工程与自然科学研究理事会;

关键词：

LARGE-PORE ZEOLITES; STRUCTURE-DIRECTING AGENTS; PILLARED MOLECULAR-SIEVE; OF-THE-ART; CRYSTAL-STRUCTURE; TOPOTACTIC CONDENSATION; LAYERED PRECURSOR; HYDROTHERMAL SYNTHESIS; MICROPOROUS ZEOLITE; CATALYTIC-ACTIVITY;

D O I：

10.1039/c5cs00045a

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A novel methodology, called ADOR (assembly-disassembly-organisation-reassembly), for the synthesis of zeolites is reviewed here in detail. The ADOR mechanism stems from the fact that certain chemical weakness against a stimulus may be present in a zeolite framework, which can then be utilized for the preparation of new solids through successive manipulation of the material. In this review, we discuss the critical factors of germanosilicate zeolites required for application of the ADOR protocol and describe the mechanism of hydrolysis, organisation and condensation to form new zeolites starting from zeolite UTL. Last but not least, we discuss the potential of this methodology to form other zeolites and the prospects for future investigations.

引用

页码：7177 / 7206

页数：30

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