High-yield fabrication of nm-size gaps in monolayer CVD graphene

被引:61
作者
Nef, Cornelia [1 ]
Posa, Laszlo [2 ,3 ]
Makk, Peter [1 ,2 ,3 ]
Fu, Wangyang [1 ]
Halbritter, Andras [2 ,3 ]
Schoenenberger, Christian [1 ]
Calame, Michel [1 ]
机构
[1] Univ Basel, Dept Phys, CH-4056 Basel, Switzerland
[2] Budapest Univ Technol & Econ, Dept Phys, H-1111 Budapest, Hungary
[3] MTA BME Condensed Matter Res Grp, H-1111 Budapest, Hungary
关键词
SINGLE MOLECULES; CONDUCTANCE; TRANSISTORS; SCATTERING; PHONONS; DEVICES;
D O I
10.1039/c4nr01838a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Herein we demonstrate the controlled and reproducible fabrication of sub-5 nm wide gaps in single-layer graphene electrodes. The process is implemented for graphene grown via chemical vapor deposition using an electroburning process at room temperature and in vacuum. A yield of over 95% for the gap formation is obtained. This approach allows producing single-layer graphene electrodes for molecular electronics at a large scale. Additionally, from Raman spectroscopy and electroburning carried out simultaneously, we can follow the heating process and infer the temperature at which the gap formation happens.
引用
收藏
页码:7249 / 7254
页数:6
相关论文
共 60 条
[1]   Patterning, Characterization, and Chemical Sensing Applications of Graphene Nanoribbon Arrays Down to 5 nm Using Helium Ion Beam Lithography [J].
Abbas, Ahmad N. ;
Liu, Gang ;
Liu, Bilu ;
Zhang, Luyao ;
Liu, He ;
Ohlberg, Douglas ;
Wu, Wei ;
Zhou, Chongwu .
ACS NANO, 2014, 8 (02) :1538-1546
[2]   Correlating Structure, Conductance, and Mechanics of Silver Atomic-Scale Contacts [J].
Aradhya, Sriharsha V. ;
Frei, Michael ;
Halbritter, Andras ;
Venkataraman, Latha .
ACS NANO, 2013, 7 (04) :3706-3712
[3]   Ballistic to diffusive crossover of heat flow in graphene ribbons [J].
Bae, Myung-Ho ;
Li, Zuanyi ;
Aksamija, Zlatan ;
Martin, Pierre N. ;
Xiong, Feng ;
Ong, Zhun-Yong ;
Knezevic, Irena ;
Pop, Eric .
NATURE COMMUNICATIONS, 2013, 4
[4]   Imaging, Simulation, and Electrostatic Control of Power Dissipation in Graphene Devices [J].
Bae, Myung-Ho ;
Ong, Zhun-Yong ;
Estrada, David ;
Pop, Eric .
NANO LETTERS, 2010, 10 (12) :4787-4793
[5]  
Balandin AA, 2011, NAT MATER, V10, P569, DOI [10.1038/nmat3064, 10.1038/NMAT3064]
[6]   ANHARMONIC EFFECTS IN LIGHT-SCATTERING DUE TO OPTICAL PHONONS IN SILICON [J].
BALKANSKI, M ;
WALLIS, RF ;
HARO, E .
PHYSICAL REVIEW B, 1983, 28 (04) :1928-1934
[7]   Graphene at High Bias: Cracking, Layer by Layer Sublimation, and Fusing [J].
Barreiro, A. ;
Boerrnert, F. ;
Ruemmeli, M. H. ;
Buechner, B. ;
Vandersypen, L. M. K. .
NANO LETTERS, 2012, 12 (04) :1873-1878
[8]   Quantum Dots at Room Temperature Carved out from Few-Layer Graphene [J].
Barreiro, Amelia ;
van der Zant, Herre S. J. ;
Vandersypen, Lieven M. K. .
NANO LETTERS, 2012, 12 (12) :6096-6100
[9]   Structured Graphene Devices for Mass Transport [J].
Barreiro, Amelia ;
Rurali, Riccardo ;
Hernandez, Eduardo R. ;
Bachtold, Adrian .
SMALL, 2011, 7 (06) :775-780
[10]   Transport Properties of Graphene in the High-Current Limit [J].
Barreiro, Amelia ;
Lazzeri, Michele ;
Moser, Joel ;
Mauri, Francesco ;
Bachtold, Adrian .
PHYSICAL REVIEW LETTERS, 2009, 103 (07)