Estimation of nocturnal222Rn soil fluxes over Russia from TROICA measurements

被引:6
作者
Berezina, E. V. [1 ]
Elansky, N. F. [1 ]
Moiseenko, K. B. [1 ]
Belikov, I. B. [1 ]
Shumsky, R. A. [1 ]
Safronov, A. N. [1 ]
Brenninkmeijer, C. A. M. [2 ]
机构
[1] Russian Acad Sci, AM Obukhov Inst Atmospher Phys, Moscow, Russia
[2] Max Planck Inst Chem, Air Chem Div, D-55128 Mainz, Germany
关键词
VERTICAL-DISTRIBUTION; ATMOSPHERIC RADON; DECAY PRODUCTS; RN-222; CONCENTRATIONS; METHANE; EXHALATION; DIFFUSION; LAYER; DUST; CO2;
D O I
10.5194/acp-13-11695-2013
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In TROICA (TRanscontinental Observations Into the Chemistry of the Atmosphere) campaigns (1999-2008), the simultaneous observations of near surface Rn-222 concentrations and atmospheric boundary layer thermal structure were performed along the Trans-Siberian Railway across northern Eurasia from Moscow to Vladivostok, including central, southern and far eastern parts of Russia. The data on Rn-222 and temperature vertical distribution are used to estimate Rn-222 regional scale soil fluxes based on calculations of nocturnal Rn-222 accumulation rates in the surface layer under inversion conditions. An effect of seasonal soil thawing on 2-4 times surface Rn-222 concentration increase from summer 1999 to autumn 2005 is observed. The estimated Rn-222 regional averaged fluxes vary over Russia from 29 +/- 8 mBq m(-2) s(-1) in its so-called European territory to 95 +/- 51 mBq m(-2) s(-1) in the southern area of Siberia. The highest Rn-222 fluxes are derived in the regions of high tectonic activity and orogenic belts of central and eastern Siberia and in far eastern Russia. The observed high Rn-222 flux variations in specific events show a strong effect of both soil and atmospheric conditions on Rn-222 near-surface abundance and the derived seasonal patterns over the continent.
引用
收藏
页码:11695 / 11708
页数:14
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