Fate of geosmin and 2-methylisoborneol in full-scale water treatment plants

被引:89
作者
Zamyadi, Arash [1 ]
Henderson, Rita [2 ]
Stuetz, Richard [1 ]
Hofmann, Ron [3 ]
Ho, Lionel [4 ]
Newcombe, Gayle [4 ]
机构
[1] Univ New S Wales, Sch Civil & Environm Engn, UNSW Water Res Ctr, Sydney, NSW 2052, Australia
[2] Univ New S Wales, Sch Chem Engn, BioMASS Lab, Sydney, NSW 2052, Australia
[3] Univ Toronto, Dept Civil Engn, Toronto, ON M5S 1A4, Canada
[4] South Australian Water Corp SA Water, Australian Water Qual Ctr AWQC, Adelaide, SA 5000, Australia
基金
澳大利亚研究理事会; 加拿大自然科学与工程研究理事会;
关键词
Cyanobacteria; Geosmin; MIB; Taste and odour; Water treatment; DRINKING-WATER; ACTIVATED CARBON; SIMULTANEOUS ADSORPTION; RAW WATER; CYANOBACTERIA; REMOVAL; TASTE; MIB; CELL; BREAKTHROUGH;
D O I
10.1016/j.watres.2015.06.038
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The increasing frequency and intensity of taste and odour (T&O) producing cyanobacteria in water sources is a growing global issue. Geosmin and 2-methylisoborneol (MIB) are the main cyanobacterial T&O compounds and can cause complaints from consumers at levels as low as 10 ng/L. However, literature concerning the performance of full-scale treatment processes for geosmin and MIB removal is rare. Hence, the objectives of this study were to: 1) estimate the accumulation and breakthrough of geosmin and MIB inside full-scale water treatment plants; 2) verify the potential impact of sludge recycling practice on performance of plants; and, 3) assess the effectiveness of aged GAC for the removal of these compounds. Sampling after full-scale treatment processes and GAC pilot assays were conducted to achieve these goals. Geosmin and MIB monitoring in full-scale plants provided the opportunity to rank the performance of studied treatment processes with filtration and granular activated carbon providing the best barriers for removal of total and extracellular compounds, correspondingly. Geosmin was removed to a greater extent than MIB using GAC. Geosmin and MIB residuals in water post GAC contactors after two years of operation was 20% and 40% of initial concentrations, correspondingly. Biological activity on the GAC surface enhanced the removal of T&O compounds. These observations demonstrated that a multi-barrier treatment approach is required to ensure cyanobacteria and their T&O compounds are effectively removed from drinking water. (C) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:171 / 183
页数:13
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