Morphology-controlled CuO nanoparticles for electroreduction of CO2 to ethanol

被引:71
作者
Chi, Dinghui [1 ]
Yang, Hengpan [1 ]
Du, Yanfang [1 ]
Lv, Ting [1 ]
Sui, Guojiao [1 ]
Wang, Huan [1 ]
Lu, Jiaxing [1 ]
机构
[1] E China Normal Univ, Dept Chem, Shanghai Key Lab Green Chem & Chem Proc, Shanghai 200062, Peoples R China
来源
RSC ADVANCES | 2014年 / 4卷 / 70期
基金
中国国家自然科学基金;
关键词
ELECTROCHEMICAL REDUCTION; 3-PHASE INTERFACE; CARBON-DIOXIDE; COPPER ELECTRODE; ETHYLENE; HYDROCARBONS; SELECTIVITY; SURFACES;
D O I
10.1039/c4ra05415f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
CuO nanoparticles with five morphologies were synthesized in large quantities using a simple method. They were in situ reduced to metallic Cu for the electroreduction of CO2. Alcohols with excellent selectivity for ethanol were obtained. The specific morphology was demonstrated to be more electrocatalytically active than others by multiple methods.
引用
收藏
页码:37329 / 37332
页数:4
相关论文
共 17 条
  • [1] Catalysis of the electrochemical reduction of carbon dioxide
    Costentin, Cyrille
    Robert, Marc
    Saveant, Jean-Michel
    [J]. CHEMICAL SOCIETY REVIEWS, 2013, 42 (06) : 2423 - 2436
  • [2] A review of the aqueous electrochemical reduction of CO2 to hydrocarbons at copper
    Gattrell, M.
    Gupta, N.
    Co, A.
    [J]. JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 2006, 594 (01) : 1 - 19
  • [3] Electrochemical conversion of CO2 to C2 hydrocarbons using different ex situ copper electrodeposits
    Goncalves, M. R.
    Gomes, A.
    Condeco, J.
    Fernandes, T. R. C.
    Pardal, T.
    Sequeira, C. A. C.
    Branco, J. B.
    [J]. ELECTROCHIMICA ACTA, 2013, 102 : 388 - 392
  • [4] Selective electrochemical conversion of CO2 to C2 hydrocarbons
    Goncalves, M. R.
    Gomes, A.
    Condeco, J.
    Fernandes, R.
    Pardal, T.
    Sequeira, C. A. C.
    Branco, J. B.
    [J]. ENERGY CONVERSION AND MANAGEMENT, 2010, 51 (01) : 30 - 32
  • [5] ELECTROCHEMICAL REDUCTION OF CO2 ON A CU ELECTRODE UNDER HIGH-PRESSURE - FACTORS THAT DETERMINE THE PRODUCT SELECTIVITY
    HARA, K
    TSUNETO, A
    KUDO, A
    SAKATA, T
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1994, 141 (08) : 2097 - 2103
  • [6] PRODUCTION OF METHANE AND ETHYLENE IN ELECTROCHEMICAL REDUCTION OF CARBON-DIOXIDE AT COPPER ELECTRODE IN AQUEOUS HYDROGENCARBONATE SOLUTION
    HORI, Y
    KIKUCHI, K
    MURATA, A
    SUZUKI, S
    [J]. CHEMISTRY LETTERS, 1986, (06) : 897 - 898
  • [7] Hori Y, 2008, MOD ASP ELECTROCHEM, P89
  • [8] Electrochemical reduction of CO at a copper electrode
    Hori, Y
    Takahashi, R
    Yoshinami, Y
    Murata, A
    [J]. JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (36): : 7075 - 7081
  • [9] Electrochemical Reduction of CO2 to CH3OH at Copper Oxide Surfaces
    Le, M.
    Ren, M.
    Zhang, Z.
    Sprunger, P. T.
    Kurtz, R. L.
    Flake, J. C.
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2011, 158 (05) : E45 - E49
  • [10] Electroreduction of carbon monoxide to liquid fuel on oxide-derived nanocrystalline copper
    Li, Christina W.
    Ciston, Jim
    Kanan, Matthew W.
    [J]. NATURE, 2014, 508 (7497) : 504 - +