Model for describing resonance-enhanced strong-field ionization with shaped ultrafast laser pulses

被引:16
作者
Lunden, William D. M. [1 ]
Sandor, Peter [1 ]
Weinacht, Thomas C. [1 ]
Rozgonyi, Tamas [2 ]
机构
[1] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA
[2] Hungarian Acad Sci, Res Ctr Nat Sci, Inst Mat & Environm Chem, H-1117 Budapest, Hungary
来源
PHYSICAL REVIEW A | 2014年 / 89卷 / 05期
基金
美国国家科学基金会;
关键词
DYNAMICS; TIME;
D O I
10.1103/PhysRevA.89.053403
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present a simple model for calculating strong-field atomic and molecular ionization dominated by Freeman resonances. Our model combines multiphoton coupling between bound states, including dynamic Stark shifts, with coupling to a discretized continuum. The simplicity of the model allows us to interpret pulse-shape-dependent strong-field ionization yields and to demonstrate the relevance of strong-field atomic or molecular phase matching to ionization, as well as bound-state population transfer. Comparison with experimental measurements demonstrates that the calculations capture the essence of the pulse-shape-dependent ionization yields.
引用
收藏
页数:8
相关论文
共 31 条
[1]   The physics of attosecond light pulses [J].
Agostini, P ;
DiMauro, LF .
REPORTS ON PROGRESS IN PHYSICS, 2004, 67 (06) :813-855
[2]  
Ammosov M. V., 1986, Soviet Physics - JETP, V64, P1191
[3]   The Multielectron Ionization Dynamics Underlying Attosecond Strong-Field Spectroscopies [J].
Boguslavskiy, Andrey E. ;
Mikosch, Jochen ;
Gijsbertsen, Arjan ;
Spanner, Michael ;
Patchkovskii, Serguei ;
Gador, Niklas ;
Vrakking, Marc J. J. ;
Stolow, Albert .
SCIENCE, 2012, 335 (6074) :1336-1340
[4]   ROLE OF THE PONDEROMOTIVE POTENTIAL IN ABOVE-THRESHOLD IONIZATION [J].
BUCKSBAUM, PH ;
FREEMAN, RR ;
BASHKANSKY, M ;
MCILRATH, TJ .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1987, 4 (05) :760-764
[5]   Transform-limited pulses are not optimal for resonant multiphoton transitions [J].
Dudovich, N ;
Dayan, B ;
Faeder, SMG ;
Silberberg, Y .
PHYSICAL REVIEW LETTERS, 2001, 86 (01) :47-50
[6]   MULTIPLE ABSORPTION OF LASER PHOTONS BY ATOMS [J].
FAISAL, FHM .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1973, 6 (04) :L89-L92
[7]   Creation of multihole molecular wave packets via strong-field ionization [J].
Geissler, Dominik ;
Rozgonyi, Tamas ;
Gonzalez-Vazquez, Jesus ;
Gonzalez, Leticia ;
Nichols, Sarah ;
Weinacht, Thomas .
PHYSICAL REVIEW A, 2010, 82 (01)
[8]   EXCITATION AND IONIZATION DYNAMICS IN SHORT-PULSE MULTIPHOTON IONIZATION [J].
GIBSON, GN ;
FREEMAN, RR ;
MCILRATH, TJ ;
MULLER, HG .
PHYSICAL REVIEW A, 1994, 49 (05) :3870-3874
[9]   DYNAMICS OF THE HIGH-INTENSITY MULTIPHOTON IONIZATION OF N2 [J].
GIBSON, GN ;
FREEMAN, RR ;
MCILRATH, TJ .
PHYSICAL REVIEW LETTERS, 1991, 67 (10) :1230-1233
[10]   Real-time observation of valence electron motion [J].
Goulielmakis, Eleftherios ;
Loh, Zhi-Heng ;
Wirth, Adrian ;
Santra, Robin ;
Rohringer, Nina ;
Yakovlev, Vladislav S. ;
Zherebtsov, Sergey ;
Pfeifer, Thomas ;
Azzeer, Abdallah M. ;
Kling, Matthias F. ;
Leone, Stephen R. ;
Krausz, Ferenc .
NATURE, 2010, 466 (7307) :739-U7