A new type of half-metallic fully compensated ferrimagnet

被引:9
作者
Semboshi, S. [1 ]
Umetsu, R. Y. [1 ,2 ,3 ]
Kawahito, Y. [4 ,5 ]
Akai, H. [6 ]
机构
[1] Tohoku Univ, Inst Mat Res, Aoba Ku, 2-1-1 Katahira, Sendai, Miyagi 9808577, Japan
[2] Tohoku Univ, Ctr Spintron Res Network, Aoba Ku, 2-1-1 Katahira, Sendai, Miyagi 9808577, Japan
[3] Ctr Sci & Innovat Spintron, Aoba Ku, 2-1-1 Katahira, Sendai, Miyagi 9808577, Japan
[4] Japan Agcy Marine Earth Sci & Technol, Res Inst Value Added Informat Generat, Kanazawa Ku, 3173-25 Showa Machi, Yokohama, Kanagawa 2360001, Japan
[5] Osaka Univ, Grad Sch Engn, Dept Appl Phys, 2-1 Yamadaoka, Suita, Osaka 5650871, Japan
[6] Univ Tokyo, Inst Solid State Phys, 5-1-5 Kashiwanoha, Kashiwa, Chiba 2778581, Japan
关键词
ELECTRONIC-STRUCTURE; MAGNETIC-PROPERTIES; TEMPERATURE; NI; MAGNETORESISTANCE; FERROMAGNETISM; APPROXIMATION; FECR2S4; FIELD; FE;
D O I
10.1038/s41598-022-14561-8
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Half-metallic fully compensated ferrimagnets (HM-FCFMs) constitute a special class of half-metals exhibiting zero magnetization at zero temperature. While there have been a number of theoretical studies predicting the existence of such materials over the last 25 years, very few of those have been synthesized and observed that they exhibit expected properties. Herein, we demonstrate that a NiAs-type hexagonal-structured (CrFe)S compound could serve as an HM-FCFM material. It has a half-metallic nature of 100% spin-polarised Fermi surfaces and yet zero magnetisation at the ground state. The magnetisation shows linear behaviour as a function of the magnetic field at temperatures below the compensation temperature (similar to 190 K). In addition, it shows a high magnetic coercivity of 3.8 Tat 300 K. These magnetic features contribute to a significant development in the application of HM-FCFMs for spintronics devices.
引用
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页数:9
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