High-quality all-inorganic CsPbBr3 single crystals prepared by a facile one-step solution growth method

被引:12
|
作者
Chen, Mingming [1 ,2 ]
Yuan, Youwen [2 ]
Liu, Yuan [2 ]
Cao, Dawei [2 ]
Xu, Chunxiang [1 ]
机构
[1] Southeast Univ, State Key Lab Bioelect, Sch Biol Sci & Med Engn, Nanjing 210096, Jiangsu, Peoples R China
[2] Jiangsu Univ, Sch Phys & Elect Engn, Dept Phys, Zhenjiang 212013, Jiangsu, Peoples R China
基金
中国博士后科学基金;
关键词
LEAD HALIDE PEROVSKITES; TRANSPORT MATERIALS; QUANTUM DOTS; SOLAR-CELLS;
D O I
10.1039/d2ra01900k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this report, a facile one-step solution growth method has been proposed to synthesize high-quality all-inorganic CsPbBr3 single crystals. High-resolution X-ray diffraction, photoluminescence (PL), and current-voltage techniques have been performed to study the properties of CsPbBr3 single crystals. The results have shown that the as-grown CsPbBr3 single crystals exhibited a narrow X-ray rocking curve with a FWHM (full width at half maximum) of 0.043 degrees, a narrow room-temperature PL spectrum with the FWHM of 18.9 nm, and extremely low density of traps (similar to 5.1 x 10(9) cm(-3)). The results shown in this work will provide a valuable strategy for the fabrication of high-quality all-inorganic CsPbBr3 single crystals.
引用
收藏
页码:14838 / 14843
页数:6
相关论文
共 35 条
  • [21] Air-stable and low threshold amplified spontaneous emission via CsBr aqueous solution processed all-inorganic CsPbBr3 perovskite films
    Liu, Ruqing
    Chen, Wei
    Liu, Li
    Lu, Yannan
    Li, Weili
    Fu, Tiliang
    Liu, Xiang
    Hang, Xiao-Chun
    Sun, Zhengyi
    APPLIED PHYSICS LETTERS, 2021, 118 (25)
  • [22] Achieving long carrier lifetime and high optical gain in all-inorganic CsPbBr3 perovskite films via top and bottom surface modification
    Jiang, Li
    Fang, Zhishan
    Lou, Haoran
    Lin, Chen
    Chen, Zhanhang
    Li, Jing
    He, Haiping
    Ye, Zhizhen
    PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2019, 21 (39) : 21996 - 22001
  • [23] Superior nonlinear optical performance of CsPbBr3 all-inorganic metal halide perovskite nano-crystals embedded Ge2S3 chalcogenide glass
    Luo, Qi
    Chen, Feifei
    Nie, Qiuhua
    Shen, Xiang
    Lin, Changgui
    Dai, Shixun
    Xu, Tiefeng
    OPTICS EXPRESS, 2025, 33 (08): : 17312 - 17324
  • [24] A Comparative Study of Light-Emitting Diodes Based on All-Inorganic Perovskite Nanoparticles (CsPbBr3) Synthesized at Room Temperature and by a Hot-Injection Method
    Clasen Hames, Bruno
    Sanchez, Rafael Sanchez
    Fakharuddin, Azhar
    Mora-Sero, Ivan
    CHEMPLUSCHEM, 2018, 83 (04): : 294 - 299
  • [25] High-efficiency Ca2+ doping all-inorganic nanocrystals (CsPbBr3 and CsPbBr1I2) encapsulated in a superhydrophobic aerogel inorganic matrix for white light-emitting diodes
    He, Ziyao
    Liang, Xiaojuan
    Xiang, Weidong
    CHEMICAL ENGINEERING JOURNAL, 2022, 427
  • [26] Nucleation-controlled growth of superior long oriented CsPbBr3 microrod single crystals for high detectivity photodetectors
    Cheng, Xiaohua
    Yuan, Ye
    Jing, Lin
    Zhou, Tianliang
    Li, Zhengxiao
    Peng, Zhiwei
    Yao, Qing
    Zhang, Jie
    Ding, Jianxu
    JOURNAL OF MATERIALS CHEMISTRY C, 2019, 7 (45) : 14188 - 14197
  • [27] 50-Fold EQE Improvement up to 6.27% of Solution-Processed All-Inorganic Perovskite CsPbBr3 QLEDs via Surface Ligand Density Control
    Li, Jianhai
    Xu, Leimeng
    Wang, Tao
    Song, Jizhong
    Chen, Jiawei
    Xue, Jie
    Dong, Yuhui
    Cai, Bo
    Shan, Qingsong
    Han, Boning
    Zeng, Haibo
    ADVANCED MATERIALS, 2017, 29 (05)
  • [28] A simple one-step method with wide processing window for high-quality perovskite mini-module fabrication
    Huang, Hsin-Hsiang
    Liu, Qi-Han
    Tsai, Hsinhan
    Shrestha, Shreetu
    Su, Li-Yun
    Chen, Po-Tuan
    Chen, Yu-Ting
    Yang, Tso-An
    Lu, Hsin
    Chuang, Ching-Hsiang
    Lin, King-Fu
    Rwei, Syang-Peng
    Nie, Wanyi
    Wang, Leeyih
    JOULE, 2021, 5 (04) : 958 - 974
  • [29] Microwave-assisted synthesis of high-quality "all-inorganic'' CsPbX3 (X = Cl, Br, I) perovskite nanocrystals and their application in light emitting diodes
    Pan, Qi
    Hu, Huicheng
    Zou, Yatao
    Chen, Min
    Wu, Linzhong
    Yang, Di
    Yuan, Xiaolei
    Fan, Jian
    Sun, Baoquan
    Zhang, Qiao
    JOURNAL OF MATERIALS CHEMISTRY C, 2017, 5 (42) : 10947 - 10954
  • [30] Mesoporous Silica Particles Integrated with All-Inorganic CsPbBr3 Perovskite Quantum-Dot Nanocomposites (MP-PQDs) with High Stability and Wide Color Gamut Used for Backlight Display
    Wang, Hung-Chia
    Lin, Shin-Ying
    Tang, An-Cih
    Singh, Bheeshma Pratap
    Tong, Hung-Chun
    Chen, Ching-Yi
    Lee, Yu-Chun
    Tsai, Tzong-Liang
    Liu, Ru-Shi
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2016, 55 (28) : 7924 - 7929