A versatile apparatus for time-resolved photoemission spectroscopy via femtosecond pump-probe experiments

被引：35

作者：

Carpene, E. ^{[1
]}

Mancini, E. ^{[1
]}

Dallera, C. ^{[1
]}

Ghiringhelli, G. ^{[2
]}

Manzoni, C. ^{[1
]}

Cerullo, G. ^{[1
]}

De Silvestri, S. ^{[1
]}

机构：

[1] Politecn Milan, CNR INFM Ultras, Dipartimento Fis, I-20133 Milan, Italy

[2] Politecn Milan, CNR INFM Coherentia & Soft, Dipartimento Fis, I-20133 Milan, Italy

来源：

REVIEW OF SCIENTIFIC INSTRUMENTS | 2009年 / 80卷 / 05期

关键词：

Auger electron spectra; copper; high-speed optical techniques; low energy electron diffraction; photoelectron spectra; silver; time resolved spectra; ULTRAFAST ELECTRON DYNAMICS; PHOTOELECTRON-SPECTROSCOPY; 2-PHOTON PHOTOEMISSION; CU(111); AG(111);

D O I：

10.1063/1.3125049

中图分类号：

TH7 [仪器、仪表];

学科分类号：

0804 ; 080401 ; 081102 ;

摘要：

A laser-based system for time-resolved photoemission spectroscopy using up to 6.2 eV photons is presented. The versatility of the laser source permits several combinations of pump and probe photon energies with pulse durations of 50-100 fs. The ultrahigh vacuum system, equipped with evaporators, a low energy electron diffraction system and an Auger spectrometer, grants the possibility to grow and characterize thin films in situ. The electron energy analyzer is a time-of-flight spectrometer with a multianode detector allowing high count rates. The performance of the whole experimental setup is investigated on Cu(100), Cu(111), and Ag(111) single crystals.

引用

页数：8

共 32 条

[1] Time-resolved pump-probe experiments beyond the jitter limitations at FLASH
Azima, A.
Duesterer, S.
Radcliffe, P.
Redlin, H.
Stojanovic, N.
Li, W.
Schlarb, H.
Feldhaus, J.
Cubaynes, D.
Meyer, M.
Dardis, J.
Hayden, P.
Hough, P.
Richardson, V.
Kennedy, E. T.
Costello, J. T.
APPLIED PHYSICS LETTERS, 2009, 94 (14)
[2] Time-resolved multi-mass ion imaging: Femtosecond UV-VUV pump-probe spectroscopy with the PImMS camera
Forbes, Ruaridh
Makhija, Varun
Veyrinas, Kevin
Stolow, Albert
Lee, Jason W. L.
Burt, Michael
Brouard, Mark
Vallance, Claire
Wilkinson, Iain
Lausten, Rune
Hockett, Paul
JOURNAL OF CHEMICAL PHYSICS, 2017, 147 (01)
[3] Calculating time-resolved differential absorbance spectra for ultrafast pump-probe experiments with surface hopping trajectories
Petit, Andrew S.
Subotnik, Joseph E.
JOURNAL OF CHEMICAL PHYSICS, 2014, 141 (15)
[4] First-principles modelling for time-resolved ARPES under different pump-probe conditions
De Giovannini, Umberto
Sato, Shunsuke A.
Hubener, Hannes
Rubio, Angel
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2022, 254
[5] Measuring correlated electron dynamics with time-resolved photoemission spectroscopy
Eckstein, Martin
Kollar, Marcus
PHYSICAL REVIEW B, 2008, 78 (24)
[6] Spectroscopy of triplet states of Rb2 by femtosecond pump-probe photoionization of doped helium nanodroplets
Mudrich, M.
Heister, Ph.
Hippler, T.
Giese, Ch.
Dulieu, O.
Stienkemeier, F.
PHYSICAL REVIEW A, 2009, 80 (04):
[7] Pump-probe photoemission simulated in real time: Revealing many-particle signatures
Hammon, Sebastian
Kuemmel, Stephan
PHYSICAL REVIEW A, 2021, 104 (01)
[8] Ultrafast carrier dynamics in Si and on Si surfaces studied by femtosecond time-resolved two-photon photoemission spectroscopy
Tanimura, K.
Ichibayashi, T.
ULTRAFAST PHENOMENA IN SEMICONDUCTORS AND NANOSTRUCTURE MATERIALS XIII, 2009, 7214
[9] On the calculation of rotational anisotropy decay, as measured by ultrafast polarization-resolved vibrational pump-probe experiments
Lin, Y. -S.
Pieniazek, P. A.
Yang, Mino
Skinner, J. L.
JOURNAL OF CHEMICAL PHYSICS, 2010, 132 (17)
[10] Femtosecond Time-Resolved Spectroscopic Photoemission Electron Microscopy for Probing Ultrafast Carrier Dynamics in Heterojunctions
Li, Bo-han
Zhang, Guan-hua
Liang, Yu
Hao, Qun-qing
Sun, Ju-long
Zhou, Chuan-yao
Tao, You-tian
Yan, Xue-ming
Ren, Ze-feng
CHINESE JOURNAL OF CHEMICAL PHYSICS, 2019, 32 (04) : 399 - 405

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