Transient IR hole burning on hydrogen-bonded liquids

被引：11

作者：

Seifert, G

Weidlich, K

Hofmann, M

Zurl, R

Graener, H

机构：

[1] UNIV HALLE WITTENBERG,FACHBEREICH PHYS FG OPT,D-06099 HALLE,GERMANY

[2] UNIV BAYREUTH,INST PHYS,LEHRSTUHL EP 3,D-95440 BAYREUTH,GERMANY

来源：

JOURNAL DE CHIMIE PHYSIQUE ET DE PHYSICO-CHIMIE BIOLOGIQUE | 1996年 / 93卷 / 10期

关键词：

vibrational spectroscopy; picosecond hole burning; molecular dynamics; thermalization;

D O I：

10.1051/jcp/1996931763

中图分类号：

Q5 [生物化学]; Q7 [分子生物学];

学科分类号：

071010 ; 081704 ;

摘要：

Transient hole burning experiments on the OH bands of hydrogen bonded liquids (ethanol/CCl4 mixtures, isotopically diluted ethanol and water) with picosecond pulses are reported and discussed. Vibrational hole burning in the Anti-Stokes Raman scattering from ethanol:CCl4 is observed for the first time. Very short effective vibrational lifetimes less than or equal to 4 ps are found in each case; a time scale of a few picoseconds is found for thermalization of the relaxed excess energy.

引用

收藏

页码：1763 / 1782

页数：20

相关论文

共 50 条

[21] Statics and Dynamics of Free and Hydrogen-Bonded OH Groups at the Air/Water Interface [J].

Verde, Ana Vila ;

Bolhuis, Peter G. ;

Campen, R. Kramer .

JOURNAL OF PHYSICAL CHEMISTRY B, 2012, 116 (31) :9467-9481

[22] The critical size of hydrogen-bonded alcohol clusters as effective Bronsted bases in solutions [J].

Park, Sun-Young ;

Kim, Taeg Gyum ;

Ajitha, Manjaly J. ;

Kwac, Kijeong ;

Lee, Young Min ;

Kim, Heesu ;

Jung, Yousung ;

Kwon, Oh-Hoon .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2016, 18 (36) :24880-24889

[23] Structure of hydrogen-bonded associates in supercritical water under low and high pressures [J].

Antipova, M. L. ;

Gurina, D. L. ;

Petrenko, V. E. .

RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A, 2013, 87 (03) :449-453

[24] Nuclear quantum effect on the hydrogen-bonded structure of guanine-cytosine pair [J].

Daido, Masashi ;

Koizumi, Akihito ;

Shiga, Motoyuki ;

Tachikawa, Masanori .

THEORETICAL CHEMISTRY ACCOUNTS, 2011, 130 (2-3) :385-391

[25] Dynamics of grain boundaries in two-dimensional hydrogen-bonded molecular networks [J].

Lackinger, M ;

Griessl, S ;

Kampschulte, L ;

Jamitzky, F ;

Heckl, WM .

SMALL, 2005, 1 (05) :532-539

[26] Tailoring carbon nitride properties and photoactivity by interfacial engineering of hydrogen-bonded frameworks [J].

Dolai, Susmita ;

Barrio, Jesus ;

Peng, Guiming ;

Grafmueller, Andrea ;

Shalom, Menny .

NANOSCALE, 2019, 11 (12) :5564-5570

[27] Hierarchically hydrogen-bonded graphene/polymer interfaces with drastically enhanced interfacial thermal conductance [J].

Zhang, Lin ;

Liu, Ling .

NANOSCALE, 2019, 11 (08) :3656-3664

[28] On similarity of hydrogen-bonded networks in liquid formamide and water as revealed in the static dielectric studies [J].

Jadzyn, Jan ;

Swiergiel, Jolanta .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2012, 14 (09) :3170-3175

[29] Cryogenic ion trap vibrational spectroscopy of hydrogen-bonded clusters relevant to atmospheric chemistry [J].

Heine, Nadja ;

Asmis, Knut R. .

INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY, 2015, 34 (01) :1-34

[30] Hydrogen-Bonded Networks Along and Bifurcation of the E-Pathway in Quinol:Fumarate Reductase [J].

Herzog, Elena ;

Gu, Wei ;

Juhnke, Hanno D. ;

Haas, Alexander H. ;

Maentele, Werner ;

Simon, Joerg ;

Helms, Volkhard ;

Lancaster, C. Roy D. .

BIOPHYSICAL JOURNAL, 2012, 103 (06) :1305-1314

← 1 2 3 4 5 →