Transient IR hole burning on hydrogen-bonded liquids

被引：11
作者：
Seifert, G
Weidlich, K
Hofmann, M
Zurl, R
Graener, H
机构：
[1] UNIV HALLE WITTENBERG,FACHBEREICH PHYS FG OPT,D-06099 HALLE,GERMANY
[2] UNIV BAYREUTH,INST PHYS,LEHRSTUHL EP 3,D-95440 BAYREUTH,GERMANY
来源：
JOURNAL DE CHIMIE PHYSIQUE ET DE PHYSICO-CHIMIE BIOLOGIQUE | 1996年 / 93卷 / 10期
关键词：
vibrational spectroscopy; picosecond hole burning; molecular dynamics; thermalization;
D O I：
10.1051/jcp/1996931763
中图分类号：
Q5 [生物化学]; Q7 [分子生物学];
学科分类号：
071010 ; 081704 ;
摘要：
Transient hole burning experiments on the OH bands of hydrogen bonded liquids (ethanol/CCl4 mixtures, isotopically diluted ethanol and water) with picosecond pulses are reported and discussed. Vibrational hole burning in the Anti-Stokes Raman scattering from ethanol:CCl4 is observed for the first time. Very short effective vibrational lifetimes less than or equal to 4 ps are found in each case; a time scale of a few picoseconds is found for thermalization of the relaxed excess energy.
引用
收藏
页码：1763 / 1782
页数：20
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