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Uneven distribution of inorganic pollutants in marine air originating from ocean-going ships
被引:13
作者:
Bencs, Laszlo
[1
,2
]
Horemans, Benjamin
[1
,3
]
Buczynska, Anna Jolanta
[1
,4
]
Van Grieken, Rene
[1
]
机构:
[1] Univ Antwerp, Dept Chem, Groenenborgerlaan 171, BE-2610 Antwerp, Belgium
[2] Hungarian Acad Sci, Wigner Res Ctr Phys, Inst Solid State Phys & Opt, POB 49, H-1525 Budapest, Hungary
[3] Univ Ghent, Fac Biosci Engn, Dept Food Safety & Food Qual, Coupure Links 653, BE-9000 Ghent, Belgium
[4] Northern Illinois Univ, Dept Geol & Environm Geosci, De Kalb, IL 60115 USA
关键词:
Ship traffic related exhaust emission;
Atmospheric pollutants;
Size-segregated aerosols;
Gaseous precursor compounds;
Secondary aerosol formation;
PARTICULATE MATTER;
EXHAUST EMISSIONS;
BOUNDARY-LAYER;
TRANSPORTATION;
PARTICLES;
QUALITY;
IMPACT;
SEA;
SO2;
D O I:
10.1016/j.envpol.2016.12.052
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
The distribution of mass, water-soluble inorganic salts and mineral elements of size-segregated aerosols (PM1, PM2.5-1 and PM10-2.5), precursor gaseous pollutants, black carbon, and nanoparticles (10-300 nm size range) at the Southern Bight of the North Sea has been studied. The concentrations of air pollutants peaked over shipping lanes, open-water anchorage areas and frequently navigated waters, due to the presence of mobile emission sources. A considerable decrease in air pollutant levels was seen when diverting from these marine areas towards remote or coastal banks. These findings showed the rapid dispersion of pollutants in the marine air. The nano-aerosol count, originating from ocean-going ships, peaked at lower average aerodynamic diameters (e.g., approximate to 28 nm) than those, observed from low displacement vessels (45-50 nm, e.g., for fishing boats). The average diameter of nano-PM depended also on weather conditions, e.g., it was higher (approximate to 50 nm) in air of higher humidity. (C) 2016 Elsevier Ltd. All rights reserved.
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页码:226 / 233
页数:8
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