Local field effects for spherical quantum dot emitters in the proximity of a planar dielectric interface

被引:9
作者
Gordon, J. M. [1 ]
Gartstein, Y. N. [1 ]
机构
[1] Univ Texas Dallas, Dept Phys, Richardson, TX 75080 USA
基金
美国国家科学基金会;
关键词
ENERGY-TRANSFER; OPTOELECTRONIC APPLICATIONS; COLLOIDAL NANOCRYSTALS; SPONTANEOUS EMISSION; PHOTOLUMINESCENCE; SENSITIZATION; BLINKING; DECAY; SI;
D O I
10.1364/JOSAB.31.002029
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We use numerical solutions of macroscopic Maxwell's equations to study spontaneous emission rates of model spherical quantum dot (QD) emitters in the vicinity of a highly polarizable dielectric substrate. It is demonstrated that extra polarization of the QD body taking place in the interfacial region may lead to appreciable deviations from the rates that would be expected under the assumption of a fixed magnitude of the effective QD transition dipole moment. Illustrations are given for both radiative and nonradiative decay processes, and potential experimental implications are discussed. (C) 2014 Optical Society of America
引用
收藏
页码:2029 / 2035
页数:7
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