Anisotropic ultrasensitive PdTe2-based phototransistor for room-temperature long-wavelength detection

被引:121
作者
Guo, Cheng [1 ,2 ]
Hu, Yibin [1 ]
Chen, Gang [1 ,2 ]
Wei, Dacheng [3 ]
Zhang, Libo [1 ,4 ]
Chen, Zhiqingzi [1 ,2 ]
Guo, Wanlong [1 ,5 ]
Xu, Huang [1 ,2 ]
Kuo, Chia-Nung [6 ]
Lue, Chin Shan [6 ]
Bo, Xiangyan [7 ]
Wan, Xiangang [7 ]
Wang, Lin [1 ,2 ]
Politano, Antonio [8 ,9 ]
Chen, Xiaoshuang [1 ,2 ,10 ]
Lu, Wei [1 ,2 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Tech Phys, State Key Lab Infrared Phys, Shanghai 200083, Peoples R China
[2] Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China
[3] Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200433, Peoples R China
[4] Donghua Univ, Dept Optoelect Sci & Engn, Shanghai 201620, Peoples R China
[5] ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
[6] Natl Cheng Kung Univ, Dept Phys, Tainan 70101, Taiwan
[7] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Dept Phys, Natl Lab Solid State Microstruct, Nanjing 210093, Peoples R China
[8] Univ Aquila, Dept Phys & Chem Sci, Via Vetoio, I-67100 Laquila, AQ, Italy
[9] CNR, IMM Ist Microelettron & Microsistemi, 8 Str 5, I-95121 Catania, Italy
[10] Univ Chinese Acad Sci, Hangzhou Inst Adv Study, Hangzhou, Peoples R China
基金
中国国家自然科学基金;
关键词
TERAHERTZ DETECTION; SEMIMETAL; STATES;
D O I
10.1126/sciadv.abb6500
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Emergent topological Dirac semimetals afford fresh pathways for optoelectronics, although device implementation has been elusive to date. Specifically, palladium ditelluride (PdTe2) combines the capabilities provided by its peculiar band structure, with topologically protected electronic states, with advantages related to the occurrence of high-mobility charge carriers and ambient stability. Here, we demonstrate large photogalvanic effects with high anisotropy at terahertz frequency in PdTe2 -based devices. A responsivity of 10 A/W and a noise-equivalent power lower than 2 pW/Hz(0.5) are achieved at room temperature, validating the suitability of PdTe2 -based devices for applications in photosensing, polarization-sensitive detection, and large-area fast imaging. Our findings open opportunities for exploring uncooled and sensitive photoelectronic devices based on topological semimetals, especially in the highly pursuit terahertz band.
引用
收藏
页数:9
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