Magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs2CuBr4

被引:12
作者
Zvyagin, S. A. [1 ]
Ozerov, M. [1 ]
Kamenskyi, D. [1 ]
Wosnitza, J. [1 ,2 ]
Krzystek, J. [3 ]
Yoshizawa, D. [4 ]
Hagiwara, M. [4 ]
Hu, Rongwei [5 ,6 ]
Ryu, Hyejin [5 ,6 ]
Petrovic, C. [5 ,6 ]
Zhitomirsky, M. E. [7 ]
机构
[1] Helmholtz Zentrum Dresden Rossendorf, Dresden High Magnet Field Lab HLD EMFL, D-01328 Dresden, Germany
[2] Tech Univ Dresden, Inst Festkorperphys, D-01062 Dresden, Germany
[3] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
[4] Osaka Univ, Grad Sch Sci, Ctr Adv High Magnet Field Sci AHMF, Toyonaka, Osaka 5600043, Japan
[5] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA
[6] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA
[7] UJF, CEA, INAC, UMR E9001,Serv Phys Stat Magnetisme & Supraconduc, F-38054 Grenoble 9, France
来源
NEW JOURNAL OF PHYSICS | 2015年 / 17卷
关键词
magnetism; frustration; spectroscopy; HIGH-FIELD ESR; RESONANCE; PHASE; ORDER;
D O I
10.1088/1367-2630/17/11/113059
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs2CuBr4. Frequency-field diagrams of ESR excitations are measured for different orientations of magnetic fields up to 25 T. We show that the substantial zero-field energy gap, Delta approximate to 9.5 K, observed in the low-temperature excitation spectrum of Cs2CuBr4, (Zvyagin et al. 2014 Phys. Rev. Lett. 112 077206) is present well above TN. Noticeably, the transition into the long-range magnetically ordered phase does not significantly affect the size of the gap, suggesting that even below TN the high-energy spin dynamics in Cs2CuBr4 is determined by short-range-order spin correlations. The experimental data are compared with results of model spin-wave-theory calculations for spin-1/2 triangular-lattice antiferromagnet.
引用
收藏
页数:7
相关论文
共 44 条
[1]   RESONATING VALENCE BONDS - NEW KIND OF INSULATOR [J].
ANDERSON, PW .
MATERIALS RESEARCH BULLETIN, 1973, 8 (02) :153-160
[2]  
ANDREEV AF, 1976, ZH EKSP TEOR FIZ+, V70, P1522
[3]   Spin liquids in frustrated magnets [J].
Balents, Leon .
NATURE, 2010, 464 (7286) :199-208
[4]   EXACT SPECTRA, SPIN SUSCEPTIBILITIES, AND ORDER-PARAMETER OF THE QUANTUM HEISENBERG-ANTIFERROMAGNET ON THE TRIANGULAR LATTICE [J].
BERNU, B ;
LECHEMINANT, P ;
LHUILLIER, C ;
PIERRE, L .
PHYSICAL REVIEW B, 1994, 50 (14) :10048-10062
[5]   HIGH-FIELD ELECTRON-SPIN-RESONANCE AND MAGNETIZATION IN THE DIMERIZED PHASE OF CUGEO3 [J].
BRILL, TM ;
BOUCHER, JP ;
VOIRON, J ;
DHALENNE, G ;
REVCOLEVSCHI, A ;
RENARD, JP .
PHYSICAL REVIEW LETTERS, 1994, 73 (11) :1545-1548
[6]   Long-range Neel order in the triangular Heisenberg model [J].
Capriotti, L ;
Trumper, AE ;
Sorella, S .
PHYSICAL REVIEW LETTERS, 1999, 82 (19) :3899-3902
[7]   Spin waves in a triangular lattice antiferromagnet: Decays, spectrum renormalization, and singularities [J].
Chernyshev, A. L. ;
Zhitomirsky, M. E. .
PHYSICAL REVIEW B, 2009, 79 (14)
[8]   Extended scattering continua characteristic of spin fractionalization in the two-dimensional frustrated quantum magnet Cs2CuCl4 observed by neutron scattering -: art. no. 134424 [J].
Coldea, R ;
Tennant, DA ;
Tylczynski, Z .
PHYSICAL REVIEW B, 2003, 68 (13)
[9]   Direct measurement of the spin Hamiltonian and observation of condensation of magnons in the 2D frustrated quantum magnet Cs2CuCl4 -: art. no. 137203 [J].
Coldea, R ;
Tennant, DA ;
Habicht, K ;
Smeibidl, P ;
Wolters, C ;
Tylczynski, Z .
PHYSICAL REVIEW LETTERS, 2002, 88 (13) :4
[10]   Experimental realization of a 2D fractional quantum spin liquid [J].
Coldea, R ;
Tennant, DA ;
Tsvelik, AM ;
Tylczynski, Z .
PHYSICAL REVIEW LETTERS, 2001, 86 (07) :1335-1338