Dzyaloshinskii-Moriya interactions and adiabatic magnetization dynamics in molecular magnets

被引:69
作者
De Raedt, H
Miyashita, S
Michielsen, K
Machida, M
机构
[1] Univ Groningen, Ctr Mat Sci, Dept Appl Phys, NL-9747 AG Groningen, Netherlands
[2] Univ Tokyo, Grad Sch Engn, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan
关键词
D O I
10.1103/PhysRevB.70.064401
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A microscopic model of the molecular magnet V-15 is used to study mechanisms for the adiabatic change of the magnetization in time-dependent magnetic fields. The effects of the Dzyaloshinskii-Moriya interaction, the most plausible source for the energy-level repulsions that lead to adiabatic changes of the magnetization, are studied in detail. We find that the energy-level repulsions that result from this interaction exhibit a strong dependence on the direction of the applied field. We also discuss the role of magnetic anisotropy in the molecule Mn-12-acetate.
引用
收藏
页码:064401 / 1
页数:12
相关论文
共 62 条
[1]  
Abramowitz M., 1964, HDB MATH FUNCTIONS
[2]   Many-spin effects and tunneling properties of magnetic molecules [J].
Al-Saqer, M ;
Dobrovitski, VV ;
Harmon, BN ;
Katsnelson, MI .
JOURNAL OF APPLIED PHYSICS, 2000, 87 (09) :6268-6270
[3]   Quantum resonance of the magnetisation in a single-crystal of Mn12-ac [J].
Barbara, B ;
Thomas, L ;
Lionti, F ;
Sulpice, A ;
Caneschi, A .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 1998, 177 :1324-1329
[4]   High-frequency EPR spectra of a molecular nanomagnet: Understanding quantum tunneling of the magnetization [J].
Barra, AL ;
Gatteschi, D ;
Sessoli, R .
PHYSICAL REVIEW B, 1997, 56 (13) :8192-8198
[5]   Effect of local Coulomb interactions on the electronic structure and exchange interactions in Mn12 magnetic molecules -: art. no. 184435 [J].
Boukhvalov, DW ;
Lichtenstein, AI ;
Dobrovitski, VV ;
Katsnelson, MI ;
Harmon, BN ;
Mazurenko, VV ;
Anisimov, VI .
PHYSICAL REVIEW B, 2002, 65 (18) :1-6
[6]   Electronic structure and exchange interactions in V15 magnetic molecules:: LDA+U results [J].
Boukhvalov, DW ;
Dobrovitski, VV ;
Katsnelson, MI ;
Lichtenstein, AI ;
Harmon, BN ;
Kögerler, P .
JOURNAL OF APPLIED PHYSICS, 2003, 93 (10) :7080-7082
[7]   ALTERNATING-CURRENT SUSCEPTIBILITY, HIGH-FIELD MAGNETIZATION, AND MILLIMETER BAND EPR EVIDENCE FOR A GROUND S = 10 STATE IN [MN12O12(CH3COO)16(H2O)4].2CH3COOH.4H2O [J].
CANESCHI, A ;
GATTESCHI, D ;
SESSOLI, R ;
BARRA, AL ;
BRUNEL, LC ;
GUILLOT, M .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1991, 113 (15) :5873-5874
[8]   Butterfly hysteresis loop and dissipative spilt reversal in the S = 1/2, V15 molecular complex [J].
Chiorescu, I ;
Wernsdorfer, W ;
Müller, A ;
Bögge, H ;
Barbara, B .
PHYSICAL REVIEW LETTERS, 2000, 84 (15) :3454-3457
[9]   Phonon-assisted tunneling in the quantum regime of Mn12 acetate [J].
Chiorescu, I ;
Giraud, R ;
Jansen, AGM ;
Caneschi, A ;
Barbara, B .
PHYSICAL REVIEW LETTERS, 2000, 85 (22) :4807-4810
[10]   Adiabatic Landau-Zener-Stuckelberg transition with or without dissipation in the low-spin molecular system V15 -: art. no. 020402 [J].
Chiorescu, I ;
Wernsdorfer, W ;
Müller, A ;
Miyashita, S ;
Barbara, B .
PHYSICAL REVIEW B, 2003, 67 (02)