Polycyclic aromatic hydrocarbons in farmland soils around main reservoirs of Jilin Province, China: occurrence, sources and potential human health risk

被引:35
作者
Chen, Yanan [1 ]
Zhang, Jiquan [1 ]
Zhang, Feng [1 ]
Li, Fengxu [1 ]
Zhou, Mo [1 ]
机构
[1] Northeast Normal Univ, Inst Nat Disaster Res, Sch Environm, Changchun 130024, Jilin, Peoples R China
基金
中国国家自然科学基金;
关键词
Polycyclic aromatic hydrocarbons (PAHs); Reservoirs; Farmland soils; Human health risk; AGRICULTURAL SOILS; SPATIAL-DISTRIBUTION; SOUTH CHINA; SOURCE APPORTIONMENT; SEASONAL-VARIATIONS; EMISSION SOURCES; RIVER ESTUARY; SURFACE SOIL; PAHS; URBAN;
D O I
10.1007/s10653-017-0024-5
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Study on the occurrence, sources and potential human health risk of polycyclic aromatic hydrocarbons in farmland soils around reservoirs is of great significance for the people drinking water security. In the present study, representative farmland soil samples around main reservoirs of Jilin Province, China, were investigated for 16 PAHs. The total concentrations of 16 priority PAHs in 32 farmland soil samples ranged from 602.12 to 1271.87 ng/g, with an arithmetic average of 877.23 ng/g, and the sum of seven carcinogenic PAH concentrations ranged from 30.07 to 710.02 ng/g, with a mean value of 229.04 ng/g. The 3-ring and 4-ring PAHs were major exist and account for 45.78 and 32.03%, respectively. Non-cancer and cancer risk of pollutants were calculated, and the results indicate that the complex PAHs in farmland soils were not considered to pose significant health effects. The isomer ratios Fla/(Fla + Pyr) and BaA/(BaA + Chr) show that the PAHs in soils were generally derived from biomass and coal combustion.
引用
收藏
页码:791 / 802
页数:12
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