Dynamics of local modes during nonradiative relaxation

被引:33
作者
Calistru, DM [1 ]
Demos, SG [1 ]
Alfano, RR [1 ]
机构
[1] CUNY,GRAD SCH,NEW YORK,NY 10031
关键词
D O I
10.1103/PhysRevLett.78.374
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The direct participation of local modes in nonradiative processes taking place in impurity-doped laser crystals is investigated using time resolved resonance Raman scattering. The measured dynamics of the highest energy Cr4+ local mode in Cr:Mg2SiO4 shows that nonradiative relaxation proceeds via transfer of the nonequilibrium local mode population generated during the transition through an electronic bottleneck, to a select number of daughter phonons, and not directly, to the phonon continuum.
引用
收藏
页码:374 / 377
页数:4
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