Concentrations and fingerprints of PAHs and PCBs adsorbed onto marine plastic debris from the Indonesian Cilacap coast and the North Atlantic gyre

被引:52
作者
Bouhroum, R. [1 ]
Boulkamh, A. [1 ]
Asia, L. [2 ]
Lebarillier, S. [2 ]
Ter Halle, A. [3 ]
Syakti, A. D. [4 ,5 ]
Doumenq, P. [2 ]
Malleret, L. [2 ]
Wong-Wah-chung, P. [2 ]
机构
[1] Univ Freres Mentouri, Lab Tech Innovantes Preservat Environnm, Constantine 1, Algeria
[2] Aix Marseille Univ, CNRS, LCE, Marseille, France
[3] Univ Paul Sabatier, Univ Toulouse, Lab IMRCP, CNRS,UMR 5623, 118 Route Narbonne, F-31062 Toulouse 9, France
[4] Jenderal Soedirman Univ, Fisheries & Marine Sci Fac, Inst Sci & Community Serv, Ctr Maritime Biosci Studies, Kampus Karangwangkal, Jl Dr Suparno 53123, Purwokerto, Indonesia
[5] Raja Ali Haji Maritime Univ, Marine Sci & Fisheries Fac, Tanjungpinang 29100, Riau Islands Pr, Indonesia
关键词
Marine plastic debris; PAHs; PCBs; Indonesian Cilacap coast; North Atlantic gyre; PERSISTENT ORGANIC POLLUTANTS; POLYCYCLIC AROMATIC-HYDROCARBONS; SYNTHETIC-POLYMERS; OPEN-OCEAN; BEACHES; MICROPLASTICS; ACCUMULATION; ENVIRONMENT; INGESTION; PHOTODEGRADATION;
D O I
10.1016/j.rsma.2019.100611
中图分类号
Q14 [生态学(生物生态学)];
学科分类号
071012 ; 0713 ;
摘要
We investigated the contamination of marine plastic debris from the Indonesian Cilacap coast and the North Atlantic gyre by polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs). The mean concentrations of 15 PAHs in gyre were 58 and 142 ng/g in polyethylene (PE) and polyethylene terephthalate (PET) debris, respectively, while PE and polypropylene (PP) Indonesian debris exhibited an average content of 552 ng/g (mainly naphthalene). The mean concentration of 61 PCBs in open ocean debris was 12.2 ng/g, while coastal debris showed a worryingly high mean value of 1.4x10(4) ng/g, with the notable presence of CB6, 101 and 173. PE gyre debris contained mostly high molecular weight PAHs such as benzo(g,h,i)perylene and indeno(1,2,3-cd)pyrene and low-chlorinated PCBs such as CB52, 77 and 105, whereas PET debris contained low molecular weight PAHs (mainly acenaphthylene and phenanthrene) and high-chlorinated PCBs such as CB204. (C) 2019 Elsevier B.V. All rights reserved.
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页数:10
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