Sensitivity of Ground-Level Ozone to NOx Emission During a High Ozone Episode in SW Poland

被引：2

作者：

Walaszek, Kinga ^{[1
]}

Kryza, Maciej ^{[1
]}

Werner, Malgorzata ^{[1
,2
]}

Ojrzynska, Hanna ^{[1
]}

机构：

[1] Univ Wroclaw, Dept Climatol & Atmosphere Protect, Wroclaw, Poland

[2] Univ Worcester, Natl Pollen & Aerobiol Res Unit, Worcester, England

来源：

AIR POLLUTION MODELING AND ITS APPLICATION XXIV | 2016年

关键词：

EUROPE; MODEL;

D O I：

10.1007/978-3-319-24478-5_56

中图分类号：

P4 [大气科学（气象学）];

学科分类号：

0706 ; 070601 ;

摘要：

Sensitivity of ozone formation to NOx and VOC emission is important in terms of implementing control strategies for photochemical pollutants, helping to determine the most effective way to limit O-3 concentrations and population exposure to high levels of O-3. In this study, the role of NOx emissions on hourly O-3 concentrations is examined in order to determine whether NOx is the driver or limiting factor of ozone formation in SW Poland in high-ozone situations. In order to assess that, four scenarios are analyzed: baseline, with no modification of the available emission inventory, a 10, 20 and 30 % decrease in anthropogenic emission of NOx. The simulations were performed for an episode with high O-3 concentrations. Both spatial and temporal changes in ozone concentrations for all scenarios have been analyzed. Preliminary results show that reducing NOx emission is associated with higher O-3 concentrations, however, further research is needed to assess the role of VOC.

引用

页码：339 / 343

页数：5

共 9 条

[1] Sensitivity of ozone and aerosols to precursor emissions in Europe [J].

Aksoyoglu, Sebnem ;

Keller, Johannes ;

Oderbolz, Daniel C. ;

Barmpadimos, Iakovos ;

Prevot, Andre S. H. ;

Baltensperger, Urs .

INTERNATIONAL JOURNAL OF ENVIRONMENT AND POLLUTION, 2012, 50 (1-4) :451-459

[2] The ERA-Interim reanalysis: configuration and performance of the data assimilation system [J].

Dee, D. P. ;

Uppala, S. M. ;

Simmons, A. J. ;

Berrisford, P. ;

Poli, P. ;

Kobayashi, S. ;

Andrae, U. ;

Balmaseda, M. A. ;

Balsamo, G. ;

Bauer, P. ;

Bechtold, P. ;

Beljaars, A. C. M. ;

van de Berg, L. ;

Bidlot, J. ;

Bormann, N. ;

Delsol, C. ;

Dragani, R. ;

Fuentes, M. ;

Geer, A. J. ;

Haimberger, L. ;

Healy, S. B. ;

Hersbach, H. ;

Holm, E. V. ;

Isaksen, L. ;

Kallberg, P. ;

Koehler, M. ;

Matricardi, M. ;

McNally, A. P. ;

Monge-Sanz, B. M. ;

Morcrette, J. -J. ;

Park, B. -K. ;

Peubey, C. ;

de Rosnay, P. ;

Tavolato, C. ;

Thepaut, J. -N. ;

Vitart, F. .

QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY, 2011, 137 (656) :553-597

[3] Analysis of UK and European NOx and VOC emission scenarios in the Defra model intercomparison exercise [J].

Derwent, Richard ;

Beevers, Sean ;

Chemel, Charles ;

Cooke, Sally ;

Francis, Xavier ;

Fraser, Andrea ;

Heal, Mathew R. ;

Kitwiroon, Nutthida ;

Lingard, Justin ;

Redington, Alison ;

Sokhi, Ranjeet ;

Vieno, Massimo .

ATMOSPHERIC ENVIRONMENT, 2014, 94 :249-257

[4] Fully coupled "online" chemistry within the WRF model [J].

Grell, GA ;

Peckham, SE ;

Schmitz, R ;

McKeen, SA ;

Frost, G ;

Skamarock, WC ;

Eder, B .

ATMOSPHERIC ENVIRONMENT, 2005, 39 (37) :6957-6975

[5]

JAROSLAWSKI J, 1993, P SOC PHOTO-OPT INS, V2047, P202, DOI 10.1117/12.163484

[6] TNO-MACC_II emission inventory; a multi-year (2003-2009) consistent high-resolution European emission inventory for air quality modelling [J].

Kuenen, J. J. P. ;

Visschedijk, A. J. H. ;

Jozwicka, M. ;

van der Gon, H. A. C. Denier .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2014, 14 (20) :10963-10976

[7]

Rozbicka K., 2015, Ann. Warsaw Univer. Life Sci. Land Reclam., V46, P247, DOI [DOI 10.2478/SGGW-2014-0020, 10.2478/sggw-2014-0020]

[8] NOx versus VOC limitation of O3 production in the Po valley:: Local and integrated view based on observations -: art. no. 8191 [J].

Spirig, C ;

Neftel, A ;

Kleinman, LI ;

Hjorth, J .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D22)

[9] Have primary emission reduction measures reduced ozone across Europe? An analysis of European rural background ozone trends 1996-2005 [J].

Wilson, R. C. ;

Fleming, Z. L. ;

Monks, P. S. ;

Clain, G. ;

Henne, S. ;

Konovalov, I. B. ;

Szopa, S. ;

Menut, L. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2012, 12 (01) :437-454

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