Sensitivity of Ground-Level Ozone to NOx Emission During a High Ozone Episode in SW Poland

被引:2
作者
Walaszek, Kinga [1 ]
Kryza, Maciej [1 ]
Werner, Malgorzata [1 ,2 ]
Ojrzynska, Hanna [1 ]
机构
[1] Univ Wroclaw, Dept Climatol & Atmosphere Protect, Wroclaw, Poland
[2] Univ Worcester, Natl Pollen & Aerobiol Res Unit, Worcester, England
来源
AIR POLLUTION MODELING AND ITS APPLICATION XXIV | 2016年
关键词
EUROPE; MODEL;
D O I
10.1007/978-3-319-24478-5_56
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Sensitivity of ozone formation to NOx and VOC emission is important in terms of implementing control strategies for photochemical pollutants, helping to determine the most effective way to limit O-3 concentrations and population exposure to high levels of O-3. In this study, the role of NOx emissions on hourly O-3 concentrations is examined in order to determine whether NOx is the driver or limiting factor of ozone formation in SW Poland in high-ozone situations. In order to assess that, four scenarios are analyzed: baseline, with no modification of the available emission inventory, a 10, 20 and 30 % decrease in anthropogenic emission of NOx. The simulations were performed for an episode with high O-3 concentrations. Both spatial and temporal changes in ozone concentrations for all scenarios have been analyzed. Preliminary results show that reducing NOx emission is associated with higher O-3 concentrations, however, further research is needed to assess the role of VOC.
引用
收藏
页码:339 / 343
页数:5
相关论文
共 9 条
[1]   Sensitivity of ozone and aerosols to precursor emissions in Europe [J].
Aksoyoglu, Sebnem ;
Keller, Johannes ;
Oderbolz, Daniel C. ;
Barmpadimos, Iakovos ;
Prevot, Andre S. H. ;
Baltensperger, Urs .
INTERNATIONAL JOURNAL OF ENVIRONMENT AND POLLUTION, 2012, 50 (1-4) :451-459
[2]   The ERA-Interim reanalysis: configuration and performance of the data assimilation system [J].
Dee, D. P. ;
Uppala, S. M. ;
Simmons, A. J. ;
Berrisford, P. ;
Poli, P. ;
Kobayashi, S. ;
Andrae, U. ;
Balmaseda, M. A. ;
Balsamo, G. ;
Bauer, P. ;
Bechtold, P. ;
Beljaars, A. C. M. ;
van de Berg, L. ;
Bidlot, J. ;
Bormann, N. ;
Delsol, C. ;
Dragani, R. ;
Fuentes, M. ;
Geer, A. J. ;
Haimberger, L. ;
Healy, S. B. ;
Hersbach, H. ;
Holm, E. V. ;
Isaksen, L. ;
Kallberg, P. ;
Koehler, M. ;
Matricardi, M. ;
McNally, A. P. ;
Monge-Sanz, B. M. ;
Morcrette, J. -J. ;
Park, B. -K. ;
Peubey, C. ;
de Rosnay, P. ;
Tavolato, C. ;
Thepaut, J. -N. ;
Vitart, F. .
QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY, 2011, 137 (656) :553-597
[3]   Analysis of UK and European NOx and VOC emission scenarios in the Defra model intercomparison exercise [J].
Derwent, Richard ;
Beevers, Sean ;
Chemel, Charles ;
Cooke, Sally ;
Francis, Xavier ;
Fraser, Andrea ;
Heal, Mathew R. ;
Kitwiroon, Nutthida ;
Lingard, Justin ;
Redington, Alison ;
Sokhi, Ranjeet ;
Vieno, Massimo .
ATMOSPHERIC ENVIRONMENT, 2014, 94 :249-257
[4]   Fully coupled "online" chemistry within the WRF model [J].
Grell, GA ;
Peckham, SE ;
Schmitz, R ;
McKeen, SA ;
Frost, G ;
Skamarock, WC ;
Eder, B .
ATMOSPHERIC ENVIRONMENT, 2005, 39 (37) :6957-6975
[5]  
JAROSLAWSKI J, 1993, P SOC PHOTO-OPT INS, V2047, P202, DOI 10.1117/12.163484
[6]   TNO-MACC_II emission inventory; a multi-year (2003-2009) consistent high-resolution European emission inventory for air quality modelling [J].
Kuenen, J. J. P. ;
Visschedijk, A. J. H. ;
Jozwicka, M. ;
van der Gon, H. A. C. Denier .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2014, 14 (20) :10963-10976
[7]  
Rozbicka K., 2015, Ann. Warsaw Univer. Life Sci. Land Reclam., V46, P247, DOI [DOI 10.2478/SGGW-2014-0020, 10.2478/sggw-2014-0020]
[8]   NOx versus VOC limitation of O3 production in the Po valley:: Local and integrated view based on observations -: art. no. 8191 [J].
Spirig, C ;
Neftel, A ;
Kleinman, LI ;
Hjorth, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D22)
[9]   Have primary emission reduction measures reduced ozone across Europe? An analysis of European rural background ozone trends 1996-2005 [J].
Wilson, R. C. ;
Fleming, Z. L. ;
Monks, P. S. ;
Clain, G. ;
Henne, S. ;
Konovalov, I. B. ;
Szopa, S. ;
Menut, L. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2012, 12 (01) :437-454