Structural Tracking of a Bimolecular Reaction in Solution by Time-Resolved X-Ray Scattering

被引：42

作者：

Haldrup, Kristoffer ^{[1
,2
]}

Christensen, Morten ^{[1
,2
]}

Cammarata, Marco ^{[3
]}

Kong, Qingyu ^{[3
]}

Wulff, Michael ^{[3
]}

Mariager, Simon O. ^{[1
,2
]}

Bechgaard, Klaus ^{[1
,2
]}

Feidenhans'l, Robert ^{[1
,2
]}

Harrit, Niels ^{[1
,2
]}

Nielsen, Martin M. ^{[1
,2
]}

机构：

[1] Univ Copenhagen, Ctr Mol Movies, Dept Chem, DK-2100 Copenhagen, Denmark

[2] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark

[3] European Synchrotron Radiat Facil, F-38043 Grenoble, France

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2009年 / 48卷 / 23期

关键词：

exciplexes; photochemistry; platinum; X-ray scattering; EXCITED-STATE; DIFFRACTION; PROBE; PUMP;

D O I：

10.1002/anie.200900741

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Molecular movies: Time-resolved X-ray scattering provides direct structural information on an electronically excited complex while it is formed in the bimolecular reaction between excited octahydrogen[tetrakis-μ-diphosphito-1 κ P:2κ P F′-diplatinate](4-) (PtPOP*) and thallium ions. In the exciplex one thallium(I) and two platinum(II) ions are found to be collinear. © 2009 Wiley-VCH Verlag GmbH & Co. KGaA.

引用

页码：4180 / 4184

页数：5

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