Weak molecular chemisorption of N2/Pt(111)

被引：8

作者：

Bruch, L. W. ^{[1
]}

Nabar, R. P. ^{[2
]}

Mavrikakis, M. ^{[2
]}

机构：

[1] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA

[2] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA

来源：

JOURNAL OF PHYSICS-CONDENSED MATTER | 2009年 / 21卷 / 26期

关键词：

NITROGEN MOLECULES; N-2; ADSORPTION; MONOLAYER; DYNAMICS; SURFACE; ENERGY; N2; POTENTIALS; SUBSTRATE;

D O I：

10.1088/0953-8984/21/26/264009

中图分类号：

O469 [凝聚态物理学];

学科分类号：

070205 ;

摘要：

The ordering in a higher-order-commensurate monolayer solid of Pt(111)-(3 x 3)-4 N-2, which has coexisting physisorbed and weakly chemisorbed N-2 species, is analyzed with model calculations. Density functional theory calculations are also used to evaluate properties of chemisorbed N-2 in a (2 x 2) unit cell on Pt(111). The relation of these results to the orientational ordering of N-2 on other metal surfaces is discussed.

引用

页数：7

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