Spatially Resolved Isotopic Source Signatures of Wetland Methane Emissions

被引:58
作者
Ganesan, A. L. [1 ]
Stell, A. C. [2 ]
Gedney, N. [3 ]
Comyn-Platt, E. [4 ]
Hayman, G. [4 ]
Rigby, M. [2 ]
Poulter, B. [5 ]
Hornibrook, E. R. C. [6 ]
机构
[1] Univ Bristol, Sch Geog Sci, Bristol, Avon, England
[2] Univ Bristol, Sch Chem, Bristol, Avon, England
[3] Hadley Ctr, Met Off, Joint Ctr Hydrometeorol Res, Wallingford, Oxon, England
[4] Ctr Ecol & Hydrol, Wallingford, Oxon, England
[5] NASA, Goddard Space Flight Ctr, Biospher Sci Lab, Greenbelt, MD USA
[6] Univ British Columbia, Dept Earth Environm & Geog Sci, Okanagan Campus, Kelowna, BC, Canada
基金
英国自然环境研究理事会;
关键词
ATMOSPHERIC METHANE; GLOBAL DISTRIBUTION; FOSSIL-FUEL; CARBON; NORTHERN; CH4; RATIOS; MODEL; BOG; TEMPERATE;
D O I
10.1002/2018GL077536
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
We present the first spatially resolved wetland delta C-13(CH4) source signature map based on data characterizing wetland ecosystems and demonstrate good agreement with wetland signatures derived from atmospheric observations. The source signature map resolves a latitudinal difference of similar to 10% between northern high-latitude (mean similar to 67.8%) and tropical (mean similar to 56.7%) wetlands and shows significant regional variations on top of the latitudinal gradient. We assess the errors in inverse modeling studies aiming to separate CH4 sources and sinks by comparing atmospheric delta C-13(CH4) derived using our spatially resolved map against the common assumption of globally uniform wetland delta C-13(CH4) signature. We find a larger interhemispheric gradient, a larger high-latitude seasonal cycle, and smaller trend over the period 2000-2012. The implication is that erroneous CH4 fluxes would be derived to compensate for the biases imposed by not utilizing spatially resolved signatures for the largest source of CH4 emissions. These biases are significant when compared to the size of observed signals. Plain Language Summary Concentrations of methane are increasing in the atmosphere. In order to understand the reasons behind such variations, carbon isotopes are used to help identify changes in emission sources and sinks. We present a new global map of the carbon isotope signature associated with wetland methane emissions, the largest global source of methane to the atmosphere. We show how this newly synthesized information can lead to more accurate understanding of the causes of variations in the amount and rate of increase of methane in the atmosphere.
引用
收藏
页码:3737 / 3745
页数:9
相关论文
共 68 条
  • [1] [Anonymous], 2009, Harmonized World Soil Database version 1.1
  • [2] [Anonymous], 722201002 RIVM
  • [3] [Anonymous], 2017, GEOSCI MODEL DEV
  • [4] REVIEW AND ASSESSMENT OF METHANE EMISSIONS FROM WETLANDS
    BARTLETT, KB
    HARRISS, RC
    [J]. CHEMOSPHERE, 1993, 26 (1-4) : 261 - 320
  • [5] Controls on CH4 emissions from a northern peatland
    Bellisario, LM
    Bubier, JL
    Moore, TR
    Chanton, JP
    [J]. GLOBAL BIOGEOCHEMICAL CYCLES, 1999, 13 (01) : 81 - 91
  • [6] Satellite chartography of atmospheric methane from SCIAMACHYon board ENVISAT:: 2.: Evaluation based on inverse model simulations
    Bergamaschi, P.
    Frankenberg, C.
    Meirink, J. F.
    Krol, M.
    Dentener, F.
    Wagner, T.
    Platt, U.
    Kaplan, J. O.
    Koerner, S.
    Heimann, M.
    Dlugokencky, E. J.
    Goede, A.
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D2)
  • [7] Contribution of anthropogenic and natural sources to atmospheric methane variability
    Bousquet, P.
    Ciais, P.
    Miller, J. B.
    Dlugokencky, E. J.
    Hauglustaine, D. A.
    Prigent, C.
    Van der Werf, G. R.
    Peylin, P.
    Brunke, E. -G.
    Carouge, C.
    Langenfelds, R. L.
    Lathiere, J.
    Papa, F.
    Ramonet, M.
    Schmidt, M.
    Steele, L. P.
    Tyler, S. C.
    White, J.
    [J]. NATURE, 2006, 443 (7110) : 439 - 443
  • [8] Isotopic Ratios of Tropical Methane Emissions by Atmospheric Measurement
    Brownlow, R.
    Lowry, D.
    Fisher, R. E.
    France, J. L.
    Lanoiselle, M.
    White, B.
    Wooster, M. J.
    Zhang, T.
    Nisbet, E. G.
    [J]. GLOBAL BIOGEOCHEMICAL CYCLES, 2017, 31 (09) : 1408 - 1419
  • [9] Burkholder J. B., Tech. Rep.
  • [10] AMAZON CAPIMS (FLOATING GRASSMATS) - A SOURCE OF C-13 ENRICHED METHANE TO THE TROPOSPHERE
    CHANTON, J
    CRILL, P
    BARTLETT, K
    MARTENS, C
    [J]. GEOPHYSICAL RESEARCH LETTERS, 1989, 16 (08) : 799 - 802