Magnetic-field-induced condensation of triplons in Han Purple pigment BaCuSi2O6 -: art. no. 087203

被引:249
作者
Jaime, M
Correa, VF
Harrison, N
Batista, CD
Kawashima, N
Kazuma, Y
Jorge, GA
Stern, R
Heinmaa, I
Zvyagin, SA
Sasago, Y
Uchinokura, K
机构
[1] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA
[2] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA
[3] Tokyo Metropolitan Univ, Dept Phys, Tokyo 1920397, Japan
[4] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina
[5] NICPB, EE-12618 Tallinn, Estonia
[6] Natl Magnet Field Lab, Tallahassee, FL 32310 USA
[7] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.93.087203
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Besides being an ancient pigment, BaCuSi2O6 is a quasi-2D magnetic insulator with a gapped spin dimer ground state. The application of strong magnetic fields closes this gap, creating a gas of bosonic spin triplet excitations. The topology of the spin lattice makes BaCuSi2O6 an ideal candidate for studying the Bose-Einstein condensation of triplet excitations as a function of the external magnetic field, which acts as a chemical potential. In agreement with quantum Monte Carlo numerical simulations, we observe a distinct lambda anomaly in the specific heat together with a maximum in the magnetic susceptibility upon cooling down to liquid helium temperatures.
引用
收藏
页码:087203 / 1
页数:4
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