Mercury in Arctic air: The long-term trend

被引:23
作者
Li, Chunsheng [1 ,2 ]
Cornett, Jack [1 ,2 ]
Willie, Scott [3 ]
Lam, Joseph [3 ]
机构
[1] Hlth Canada, Radiat Protect Bur, Ottawa, ON K1A 1C1, Canada
[2] Trent Univ, Environm & Resources Studies Program, Peterborough, ON K9J 7B8, Canada
[3] Natl Res Council Canada, Inst Natl Measurement Stand, Ottawa, ON K1A 0R6, Canada
关键词
Mercury; Particulate mercury; Time trend; Arctic; Air pollution; ATMOSPHERIC MERCURY; ENVIRONMENT; DEPOSITION; GREENLAND; CANADA; ALERT; GEM;
D O I
10.1016/j.scitotenv.2008.12.010
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The long-term (1974-2000) time trend of total filterable mercury (TFM) in the air in the Canadian Arctic is reported. The concentration of TFM had declined by (3.0 +/- 0.8)% and (3.1 +/- 0.9)% per year in the summer and fall, respectively, over the 27 years, which coincided with the calculated reduction rate of world-wide mercury emission (similar to 3.3% per year) from human activities between 1983 and 1995. The time trend for winter and early spring was not statistically significant as the variability of TFM was very large, partly due to Arctic Mercury Depletion Events and partly due to Arctic haze. Crown Copyright (C) 2008 Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:2756 / 2759
页数:4
相关论文
共 22 条
[11]   Annual time-series of total filterable atmospheric mercury concentrations in the Arctic [J].
Lu, JY ;
Schroeder, WH .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2004, 56 (03) :213-222
[12]   QUANTITATIVE ASSESSMENT OF WORLDWIDE CONTAMINATION OF AIR, WATER AND SOILS BY TRACE-METALS [J].
NRIAGU, JO ;
PACYNA, JM .
NATURE, 1988, 333 (6169) :134-139
[13]   European emissions of atmospheric mercury from anthropogenic sources in 1995 [J].
Pacyna, EG ;
Pacyna, JM ;
Pirrone, N .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (17) :2987-2996
[14]  
Pacyna J.M., 2001, Environmental Reviews, V9, P269, DOI [10.1139/er-9-4-269, DOI 10.1139/A01-012]
[15]  
Pirrone N, 1996, WATER AIR SOIL POLL, V88, P145
[16]   Arctic springtime depletion of mercury [J].
Schroeder, WH ;
Anlauf, KG ;
Barrie, LA ;
Lu, JY ;
Steffen, A ;
Schneeberger, DR ;
Berg, T .
NATURE, 1998, 394 (6691) :331-332
[17]   INDICATION OF CHANGE IN GLOBAL AND REGIONAL TRENDS OF ATMOSPHERIC MERCURY CONCENTRATIONS [J].
SLEMR, F ;
JUNKERMANN, W ;
SCHMIDT, RWH ;
SLADKOVIC, R .
GEOPHYSICAL RESEARCH LETTERS, 1995, 22 (16) :2143-2146
[18]   INCREASE IN GLOBAL ATMOSPHERIC CONCENTRATIONS OF MERCURY INFERRED FROM MEASUREMENTS OVER THE ATLANTIC-OCEAN [J].
SLEMR, F ;
LANGER, E .
NATURE, 1992, 355 (6359) :434-437
[19]   Mercury in the Arctic atmosphere: An analysis of eight years of measurements of GEM at Alert (Canada) and a comparison with observations at Amderma (Russia) and Kuujjuarapik (Canada) [J].
Steffen, A ;
Schroeder, W ;
Macdonald, R ;
Poissant, L ;
Konoplev, A .
SCIENCE OF THE TOTAL ENVIRONMENT, 2005, 342 (1-3) :185-198
[20]   Environment - Uncertain science underlies new mercury standards [J].
Stokstad, E .
SCIENCE, 2004, 303 (5654) :34-34