Fe-BEA Zeolite Catalysts for NH3-SCR of NOx

被引:56
|
作者
Frey, Anne Mette [1 ]
Mert, Selcuk [1 ]
Due-Hansen, Johannes [1 ]
Fehrmann, Rasmus [1 ]
Christensen, Claus Hviid [2 ]
机构
[1] Tech Univ Denmark, Ctr Sustainable & Green Chem, Dept Chem, DK-2800 Lyngby, Denmark
[2] Haldor Topsoe Res Labs, DK-2800 Lyngby, Denmark
基金
新加坡国家研究基金会;
关键词
NH3-SCR; NOx; Fe-BEA; Zeolite catalysts; SELECTIVE REDUCTION; BETA CATALYSTS; NITRIC-OXIDE; AMMONIA; IRON; FE-ZSM-5; NH3; SPECTROSCOPY; CRYSTALS; VEHICLES;
D O I
10.1007/s10562-009-9894-1
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Iron-containing zeolites are known to be promising catalysts for the NH3-SCR reaction. Here, we will investigate the catalytic activity of iron-based BEA catalysts, which was found to exhibit improved activities compared to previously described iron-containing zeolite catalysts, such as ZSM-5 and ZSM-12. Series of Fe-BEA zeolite catalysts were prepared using a range of different preparation methods. Furthermore, we found that an iron concentration around 3 wt% on BEA showed a small optimum in SCR activity compared to the other iron loadings studied.
引用
收藏
页码:1 / 8
页数:8
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