Molecular theory of second-order sum-frequency generation

被引：28
作者：
Lin, SH
Hayashi, M
Islampour, R
Yu, J
Yang, DY
Wu, GYC
机构：
[1] ARIZONA STATE UNIV,DEPT CHEM,TEMPE,AZ 85287
[2] UNIV TEACHER EDUC,DEPT CHEM,TEHRAN,IRAN
[3] UNIV CHINESE CULTURE,DEPT CHEM,TAIPEI,TAIWAN
[4] ARIZONA STATE UNIV,CTR STUDY EARLY EVENTS PHOTOSYNTH,TEMPE,AZ 85287
来源：
PHYSICA B | 1996年 / 222卷 / 1-3期
关键词：
D O I：
10.1016/0921-4526(96)00008-7
中图分类号：
O469 [凝聚态物理学];
学科分类号：
070205 ;
摘要：
Recently the second-order sum-frequency generation (SFG) has become a powerful surface - spectroscopic technique. In this paper we present a molecular theory for SFG. To systematically treat this process, we have classified SFG into the resonance-resonance case, resonance-off-resonance case, off-resonance-resonance case and off-resonance-off-resonance case. Among these cases we may have IR-UV SFG and UV-UV SFG. Some of these SFG's are reported in this paper. In each SFG case, we have shown how to calculate the strength (or intensity) and band-shape function.
引用
收藏
页码：191 / 208
页数：18
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