Narrow-band coherent Rayleigh scattering

被引：12
|
作者：
Bookey, H. T.
Bishop, A. I.
Shneider, M. N.
Barker, P. F.
机构：
[1] Heriot Watt Univ, Sch Engn & Phys Sci, Edinburgh EH14 4AS, Midlothian, Scotland
[2] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA
来源：
JOURNAL OF RAMAN SPECTROSCOPY | 2006年 / 37卷 / 06期
关键词：
coherent Rayleigh scattering; high resolution;
D O I：
10.1002/jrs.1531
中图分类号：
O433 [光谱学];
学科分类号：
0703 ; 070302 ;
摘要：
We describe the first implementation of narrow-band coherent Rayleigh scattering (CRS) for high spectral resolution of CRS line shapes. Using intensities in the 10(9) W/cm(2) range we find that the measured line shapes Of CO2, N-2 and Xe gases at room temperature are in good agreement with a CRS model that assumes weakly perturbing fields. We compare our results with broadband CRS and discuss the importance of phase-matching requirements for narrow-band CRS. Finally, we show that a spectral narrowing in the CRS profile is predicted at intensities that are approximately an order of magnitude greater than those used in our experiments. Copyright (c) 2006 John Wiley & Sons, Ltd.
引用
收藏
页码：655 / 662
页数：8
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