Disparities between experimental and environmental conditions: Research steps toward making electrochemical water treatment a reality

被引:115
作者
Garcia-Segura, Sergi [1 ,2 ]
Nienhauser, Alec Brockway [1 ,2 ]
Fajardo, Ana S. [1 ,2 ,3 ]
Bansal, Rishabh [1 ,2 ]
Coonrod, Christian L. [1 ,4 ]
Fortner, John D. [1 ,5 ]
Marcos-Hernandez, Mariana [1 ,6 ]
Rogers, Tanya [1 ,4 ]
Villagran, Dino [1 ,6 ]
Wong, Michael S. [1 ,4 ]
Westerhoff, Paul [1 ,2 ]
机构
[1] Nanosyst Engn Res Ctr Nanotechnol Enabled Water T, Tempe, AZ USA
[2] Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA
[3] Sorbonne Univ, CNRS, Lab Interfaces & Syst Electrochim LISE, 4 Pl Jussieu, F-75005 Paris, France
[4] Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA
[5] Yale Univ, Dept Chem & Environm Engn, New Haven, CT 06520 USA
[6] Univ Texas El Paso, Dept Chem & Biochem, El Paso, TX 79968 USA
基金
美国国家科学基金会;
关键词
Electrocatalytic water treatment; Electrochemical advanced reduction processes; Electrochemical advanced oxidation processes; Borondoped diamond electrode; Magneli Ti4O7; Persistent organic pollutants; Oxyanions; BORON-DOPED DIAMOND; WASTE-WATER; ADVANCED OXIDATION; PERFLUOROOCTANOIC ACID; ORGANIC CONTAMINANTS; OPERATING PARAMETERS; ANODIC-OXIDATION; FENTON TREATMENT; ELECTRO-FENTON; FREE CHLORINE;
D O I
10.1016/j.coelec.2020.03.001
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Electrochemical water treatment is one of the key topics of environmental electrochemistry. Identifying electrocatalytic materials capable of electrogenerating high oxidant species in situ seems to have catalyzed researchers' interest in these processes. While most studies have focused on ideal lab -made solutions, translation to higher technology readiness levels and commercialization requires reframing research questions in context of real water matrices. In this current opinion, we discuss disconnects that may occur when focusing on synthetic solution treatment rather than on real waters. Future research can fill the gaps identified herein, thus facilitating application of electrochemical water treatment
引用
收藏
页码:9 / 16
页数:8
相关论文
共 79 条
[1]   Simultaneous Adsorption and Electrochemical Reduction of N-Nitrosodimethylamine Using Carbon-Ti4O7 Composite Reactive Electrochemical Membranes [J].
Almassi, Soroush ;
Li, Zhao ;
Xu, Wenqing ;
Pu, Changcheng ;
Zeng, Teng ;
Chaplin, Brian P. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2019, 53 (02) :928-937
[2]   Photoelectrocatalytic decolorization of azo dyes with nano-composite oxide layers of ZnO nanorods decorated with Ag nanoparticles [J].
Antonio Cerron-Calle, Gabriel ;
Aranda-Aguirre, Alejandro Junior ;
Luyo, Clemente ;
Garcia-Segura, Sergi ;
Alarcon, Hugo .
CHEMOSPHERE, 2019, 219 :296-304
[3]   Enhanced degradation of the antibiotic tetracycline by heterogeneous electro-Fenton with pyrite catalysis [J].
Barhoumi, Natija ;
Oturan, Nihal ;
Ammar, Salah ;
Gadri, Abdellatif ;
Oturan, Mehmet A. ;
Brillas, Enric .
ENVIRONMENTAL CHEMISTRY LETTERS, 2017, 15 (04) :689-693
[4]   Product and by-product formation in laboratory studies on disinfection electrolysis of water using boron-doped diamond anodes [J].
Bergmann, M. E. Henry ;
Rollin, Johanna .
CATALYSIS TODAY, 2007, 124 (3-4) :198-203
[5]   The occurrence of perchlorate during drinking water electrolysis using BDD anodes [J].
Bergmann, M. E. Henry ;
Rollin, Johanna ;
Iourtchouk, Tatiana .
ELECTROCHIMICA ACTA, 2009, 54 (07) :2102-2107
[6]   Combination of photoelectrocatalysis and ozonation: A novel and powerful approach applied in Acid Yellow 1 mineralization [J].
Bessegato, Guilherme Garcia ;
Cardoso, Juliano Carvalho ;
da Silva, Bianca Ferreira ;
Boldrin Zanoni, Maria Valnice .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2016, 180 :161-168
[7]   Figures-of-merit for the technical development and application of advanced oxidation technologies for both electric- and solar-driven systems - (IUPAC Technical Report) [J].
Bolton, JR ;
Bircher, KG ;
Tumas, W ;
Tolman, CA .
PURE AND APPLIED CHEMISTRY, 2001, 73 (04) :627-637
[8]   Spatial distribution and temporal trends of pharmaceuticals sorbed to suspended particulate matter of German rivers [J].
Boulard, Lise ;
Dierkes, Georg ;
Schluesener, Michael P. ;
Wick, Arne ;
Koschorreck, Jan ;
Ternes, Thomas A. .
WATER RESEARCH, 2020, 171
[9]   Benchmarking recent advances and innovative technology approaches of Fenton, photo-Fenton, electro-Fenton, and related processes: A review on the relevance of phenol as model molecule [J].
Brillas, Enric ;
Garcia-Segura, Sergi .
SEPARATION AND PURIFICATION TECHNOLOGY, 2020, 237
[10]   Indirect electrochemical oxidation of 2,4-dichlorophenoxyacetic acid using electrochemically-generated persulfate [J].
Cai, Jingju ;
Zhou, Minghua ;
Liu, Ye ;
Savall, Andre ;
Serrano, Karine Groenen .
CHEMOSPHERE, 2018, 204 :163-169