Second-harmonic Rayleigh scattering from a sphere of centrosymmetric material

被引：417
作者：
Dadap, JI
Shan, J
Eisenthal, KB
Heinz, TF
机构：
[1] Columbia Univ, Dept Phys, New York, NY 10027 USA
[2] Columbia Univ, Dept Chem, New York, NY 10027 USA
来源：
PHYSICAL REVIEW LETTERS | 1999年 / 83卷 / 20期
关键词：
D O I：
10.1103/PhysRevLett.83.4045
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We describe the electromagnetic theory of second-harmonic generation from the surface of a sphere that is small compared to the wavelength of light. In a leading-order expansion, the second-harmonic radiation is emitted in nonlocally excited electric dipole and locally excited electric quadrupole modes. We analyze the problem with particular emphasis on experimental aspects, such as the radiation pattern, polarization selection rules, determination of nonlinear susceptibilities, radiation efficiency, and spectral characteristics.
引用
收藏
页码：4045 / 4048
页数：4
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