Combinational Synthetic Approaches for Isoreticular and Polymorphic Metal-Organic Frameworks with Tuned Pore Geometries and Surface Properties

被引：38

作者：

Jeong, Seok ^{[1
]}

Kim, Dongwook ^{[1
]}

Shin, Sunyoung ^{[1
]}

Moon, Dohyun ^{[2
]}

Cho, Sung June ^{[3
,4
]}

Lah, Myoung Soo ^{[1
]}

机构：

[1] Ulsan Natl Inst Sci & Technol, Dept Chem, Ulsan 689805, South Korea

[2] Pohang Accelerator Lab, Pohang 790784, South Korea

[3] Chonnam Natl Univ, Dept Appl Chem Engn, Kwangju 500757, South Korea

[4] Chonnam Natl Univ, Res Inst Catalysis, Kwangju 500757, South Korea

来源：

CHEMISTRY OF MATERIALS | 2014年 / 26卷 / 04期

基金：

新加坡国家研究基金会;

关键词：

CARBON-DIOXIDE CAPTURE; LIGAND-EXCHANGE; POSTSYNTHETIC LIGAND; SINGLE-CRYSTAL; CO2; BINDING; ADSORPTION; STORAGE; GAS; ROUTE; IONS;

D O I：

10.1021/cm404239s

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Isoreticular and polymorphic 3-D MOFs were prepared via the combination of direct solvothermal reactions, postsynthetic ligand exchanges of the MOFs prepared via the direct solvothermal reactions, and postsynthetic ligand insertions into a 2-D MOF. The appropriate pore dimensions, surface areas, and adsorption enthalpies of the MOFs combined well to produce the largest working CO2 capture capacities via the pressure swing adsorption process.

引用

页码：1711 / 1719

页数：9

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