Combinational Synthetic Approaches for Isoreticular and Polymorphic Metal-Organic Frameworks with Tuned Pore Geometries and Surface Properties

被引：39

作者：

Jeong, Seok ^{[1
]}

Kim, Dongwook ^{[1
]}

Shin, Sunyoung ^{[1
]}

Moon, Dohyun ^{[2
]}

Cho, Sung June ^{[3
,4
]}

Lah, Myoung Soo ^{[1
]}

机构：

[1] Ulsan Natl Inst Sci & Technol, Dept Chem, Ulsan 689805, South Korea

[2] Pohang Accelerator Lab, Pohang 790784, South Korea

[3] Chonnam Natl Univ, Dept Appl Chem Engn, Kwangju 500757, South Korea

[4] Chonnam Natl Univ, Res Inst Catalysis, Kwangju 500757, South Korea

来源：

CHEMISTRY OF MATERIALS | 2014年 / 26卷 / 04期

基金：

新加坡国家研究基金会;

关键词：

CARBON-DIOXIDE CAPTURE; LIGAND-EXCHANGE; POSTSYNTHETIC LIGAND; SINGLE-CRYSTAL; CO2; BINDING; ADSORPTION; STORAGE; GAS; ROUTE; IONS;

D O I：

10.1021/cm404239s

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Isoreticular and polymorphic 3-D MOFs were prepared via the combination of direct solvothermal reactions, postsynthetic ligand exchanges of the MOFs prepared via the direct solvothermal reactions, and postsynthetic ligand insertions into a 2-D MOF. The appropriate pore dimensions, surface areas, and adsorption enthalpies of the MOFs combined well to produce the largest working CO2 capture capacities via the pressure swing adsorption process.

引用

收藏

页码：1711 / 1719

页数：9

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