Modification of acid supports by solid-state redox reaction - Part II. Acid and catalytic properties

被引:13
作者
Hagen, A
Schneider, E
Benter, M
Krogh, A
Kleinert, A
Roessner, F
机构
[1] Tech Univ Denmark, Dept Chem, Interdisciplinary Res Ctr Catal, DK-2800 Lyngby, Denmark
[2] Riso Natl Lab, Mat Res Dept, DK-4000 Roskilde, Denmark
[3] Carl V Ossietzky Univ Oldenburg, Inst Pure & Appl Chem, D-26111 Oldenburg, Germany
关键词
solid-state redox reaction; zeolite; TPAD; ethane; cyclohexane;
D O I
10.1016/j.jcat.2004.05.027
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
ZSM-5 and Y zeolites, gamma-alumina, and silica modified by solid-state redox reaction with zinc, gallium, manganese, and iron were studied in the conversion of cyclohexane and the nonoxidative conversion of ethane. The catalytic behavior was related to acid properties characterized by temperature-programmed desorption of ammonia (TPAD). (C) 2004 Elsevier Inc. All rights reserved.
引用
收藏
页码:171 / 182
页数:12
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