Tetraphenylethylene-based phosphine: tuneable emission and carbon dioxide fixation

被引：28

作者：

Zhang, Jianyong ^{[1
]}

Yang, Qiuti ^{[1
]}

Zhu, Yixuan ^{[1
]}

Liu, Haoliang ^{[1
]}

Chi, Zhenguo ^{[1
]}

Su, Cheng-Yong ^{[1
]}

机构：

[1] Sun Yat Sen Univ, Sch Chem & Chem Engn, KLGHEI Environm & Energy Chem, MOE Key Lab Polymer Composite & Funct Mat, Guangzhou 510275, Guangdong, Peoples R China

来源：

DALTON TRANSACTIONS | 2014年 / 43卷 / 42期

关键词：

METAL-ORGANIC FRAMEWORKS; AGGREGATION-INDUCED EMISSION; TURN-ON FLUORESCENCE; ATMOSPHERIC CO2 FIXATION; FUNCTIONALIZED TETRAPHENYLETHENE; COPPER(II) COMPLEXES; ENHANCED EMISSION; CLUSTERS; BINDING; LIGANDS;

D O I：

10.1039/c4dt01808g

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

A tetraphenylethylene-based phosphine, 1,1,2,2-tetrakis((4-diphenyiphosphino)phenypethylene (TPE-P4), was synthesized and showed novel aggregation-induced and mechano-responsive emission. A mixture of TPE-P4 and Ag+ could fix atmospheric CO2 in situ as carbonate ions in neutral solution to yield a rare 3D metal-organic framework with zeolite-like SOD topology, [Ag-2(TPE-P-4)CO3](x), superset of nH(2)O (Ag-TPE-P4). Ag-TPE-P4 showed turn-on luminescence of TPE-P4, emitting bright bluish green light in the solid state.

引用

页码：15785 / 15790

页数：6

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