Is there a fractional breakdown of the Stokes-Einstein relation in kinetically constrained models at low temperature?

被引:10
作者
Blondel, O. [1 ]
Toninelli, C. [1 ]
机构
[1] Univ Paris VI VII, CNRS UMR 7599, LPMA, F-75205 Paris 13, France
基金
中国国家自然科学基金;
关键词
SPATIALLY HETEROGENEOUS DYNAMICS; SUPERCOOLED O-TERPHENYL; GLASS-TRANSITION; SELF-DIFFUSION; ISING-MODEL; EAST MODEL; LIQUIDS; TIME; SCALE; SPACE;
D O I
10.1209/0295-5075/107/26005
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We study the motion of a tracer particle injected in facilitated models which are used to model supercooled liquids in the vicinity of the glass transition. We consider the East model, FA1f model and a more general class of non-cooperative models. For East previous works had identified a fractional violation of the Stokes-Einstein relation with a decoupling between diffusion and viscosity of the form D similar to tau(-xi) with xi similar to 0.73. We present rigorous results proving that instead log(D) = - log(tau) + O(log(1/q)), which implies at leading order log(D)/log(tau) similar to -1 for very large time scales. Our results do not exclude the possibility of SE breakdown, albeit non-fractional. Indeed extended numerical simulations by other authors show the occurrence of this violation and our result suggests D tau similar to 1/q(alpha), where q is the density of excitations. For FA1f we prove a fractional Stokes-Einstein relation in dimension 1, and D similar to tau(-1) in dimension 2 and higher, confirming previous works. Our results extend to a larger class of non-cooperative models. Copyright (C) EPLA, 2014
引用
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页数:6
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