Nodal ground states and orbital textures in semiconductor quantum dots

被引:10
作者
Lee, Jeongsu [1 ]
Vyborny, Karel [1 ,2 ]
Han, Jong E. [1 ]
Zutic, Igor [1 ]
机构
[1] SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA
[2] Acad Sci Czech Republ, Inst Phys, Vvi, CZ-16253 Prague 6, Czech Republic
基金
美国国家科学基金会;
关键词
ELECTRONIC-STRUCTURE CALCULATIONS; VALENCE BANDS; EXCITON; RESONANCE; DONOR; DARK;
D O I
10.1103/PhysRevB.89.045315
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Conventional understanding implies that the ground state of a nonmagnetic quantum mechanical system should be nodeless. While this notion also provides a valuable guidance in understanding the ordering of energy levels in semiconductor nanostructures, there are reports that nodal ground states for holes are possible. However, the existence of such nodal states has been debated and even viewed merely as an artifact of a k.p model. Using complementary approaches of both k.p and tight-binding models, further supported by an effective Hamiltonian for a continuum model, we reveal that nodal ground states in quantum dots are not limited to a specific approach. Remarkably, the emergence of nodal hole states at the top of the valence band can be attributed to the formation of orbital vortex textures through competition between the hole kinetic energy and the coupling to the conduction band states. We suggest an experimental test for our predictions of the reversed energy ordering and the existence of nodal ground states. We discuss how our findings and the studies of orbital textures could be also relevant for other materials systems.
引用
收藏
页数:17
相关论文
共 67 条
[1]   Theory of magnetic anisotropy in III1-xMnxV ferromagnets -: art. no. 054418 [J].
Abolfath, M ;
Jungwirth, T ;
Brum, J ;
MacDonald, AH .
PHYSICAL REVIEW B, 2001, 63 (05)
[2]   Piezomagnetic Quantum Dots [J].
Abolfath, Ramin M. ;
Petukhov, A. G. ;
Zutic, Igor .
PHYSICAL REVIEW LETTERS, 2008, 101 (20)
[3]  
[Anonymous], COMMUNICATION
[4]  
[Anonymous], 1953, METHODS THEORETICAL
[5]   Dark and bright excitonic states in nitride quantum dots [J].
Bagga, A ;
Chattopadhyay, PK ;
Ghosh, S .
PHYSICAL REVIEW B, 2005, 71 (11)
[6]   Energy levels of nitride quantum dots: Wurtzite versus zinc-blende structure [J].
Bagga, A ;
Chattopadhyay, PK ;
Ghosh, S .
PHYSICAL REVIEW B, 2003, 68 (15)
[7]   Origin of Stokes shift in InAs and CdSe quantum dots: Exchange splitting of excitonic states [J].
Bagga, Anjana ;
Chattopadhyay, P. K. ;
Ghosh, Subhasis .
PHYSICAL REVIEW B, 2006, 74 (03)
[8]   SPHERICAL MODEL OF SHALLOW ACCEPTOR STATES IN SEMICONDUCTORS [J].
BALDERESCHI, A ;
LIPARI, NO .
PHYSICAL REVIEW B, 1973, 8 (06) :2697-2709
[9]  
Bastard G., 1991, Wave Mechanics Applied to Semiconductor Heterostructures
[10]   Light-Induced Spontaneous Magnetization in Doped Colloidal Quantum Dots [J].
Beaulac, Remi ;
Schneider, Lars ;
Archer, Paul I. ;
Bacher, Gerd ;
Gamelin, Daniel R. .
SCIENCE, 2009, 325 (5943) :973-976