Synthesis ofFe2O3/TiO2/graphene aerogel composite as an efficient Fenton-photocatalyst for removal of methylene blue from aqueous solution

被引:11
作者
Tran Hoang Tu [1 ,3 ]
Le Tan Tai [1 ,3 ]
Nguyen Tan Tien [1 ]
Le Minh Huong [2 ,3 ]
Doan Thi Yen Oanh [4 ]
Hoang Minh Nam [1 ,2 ,3 ]
Mai Thanh Phong [2 ,3 ]
Nguyen Huu Hieu [1 ,2 ,3 ]
机构
[1] Ho Chi Minh City Univ Technol, Key Lab Chem Engn & Petr Proc, VNU HCM, CEPP Lab, 268 Ly Thuong Kiet St,Dist 10, Ho Chi Minh City 70000, Vietnam
[2] Ho Chi Minh City Univ Technol, Fac Chem Engn, 268 Ly Thuong Kiet St,Dist 10, Ho Chi Minh City 70000, Vietnam
[3] Vietnam Acad Sci & Technol, 6 Linh Trung Ward, Ho Chi Minh City 70000, Vietnam
[4] Vietnam Acad Sci & Technol, Publishing House Sci & Technol, 18 Hoang Quoc Viet, Hanoi 10000, Vietnam
关键词
Fe2O3; TiO2; Graphene aerogel; nanocomposite; photocatalysis; methylene blue; ORGANIC POLLUTANTS; TITANIUM-DIOXIDE; DEGRADATION; OXIDE; PHOTODEGRADATION;
D O I
10.1002/vjch.202000109
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In the present study, the composites including Fe2O3/TiO2/graphene aerogel (Fe2O3/TiO2/GA) and TiO2/graphene aerogel (TiO2/GA), and graphene aerogel (GA) were synthesized by hydrothermal method. The as-prepared materials were characterized using X-ray diffraction, Fourier transform infrared spectroscopy, scanning electron microscopy, energy dispersive X-ray, Raman spectroscopy. The characterization results showed that the Fe(2)O(3)and TiO(2)particles were uniformly attached in GA structure, increasing number of active sites of materials and extending the light absorption range. The removal performance of Fe2O3/TiO2/GA is 97.38 % which is higher than of TiO2/GA and TiO2. The degradation data were well consisted withpseudo-first-orderkinetic model. Accordingly, Fe2O3/TiO2/GA is potential to be used as an efficient photocatalysis for treatment of MB from water.
引用
收藏
页码:697 / 704
页数:8
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