Ultrasharp Lateral p-n Junctions in Modulation-Doped Graphene br

被引:22
作者
Balgley, Jesse [1 ]
Butler, Jackson [1 ]
Biswas, Sananda [2 ]
Ge, Zhehao [3 ]
Lagasse, Samuel [4 ]
Taniguchi, Takashi [5 ]
Watanabe, Kenji [6 ]
Cothrine, Matthew [7 ]
Mandrus, David G. [7 ,8 ]
Velasco, Jairo, Jr. [3 ]
Valenti, Roser [2 ]
Henriksen, Erik A. [1 ]
机构
[1] Washington Univ, Dept Phys, St Louis, MO 63130 USA
[2] Goethe Univ Frankfurt, Inst Theoret Phys, D-60438 Frankfurt, Germany
[3] UC Santa Cruz, Phys Dept, Santa Cruz, CA 95064 USA
[4] US Navy, Res Lab, Elect Sci & Technol Div, Washington, DC 20375 USA
[5] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan
[6] Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Ibaraki 3050044, Japan
[7] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA
[8] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA
基金
美国国家科学基金会;
关键词
Graphene; -RuCl3; p-n junction; electronic transport; scanning tunneling microscopy; density functional theory; DIRAC FERMIONS; OPTICS;
D O I
10.1021/acs.nanolett.2c00785
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We demonstrate ultrasharp (less than or similar to 10 nm) lateral p-n junctions in graphene using electronic transport, scanningtunneling microscopy, andfirst-principles calculations. The p-n junction lies at the boundary between differentially doped regionsof a graphene sheet, where one side is intrinsic and the other ischarge-doped by proximity to aflake of alpha-RuCl3across a thininsulating barrier. We extract the p-n junction contribution to thedevice resistance to place bounds on the junction width. Weachieve an ultrasharp junction when the boundary between theintrinsic and doped regions is defined by a cleaved crystalline edgeof alpha-RuCl3located 2 nm from the graphene. Scanning tunnelingspectroscopy in heterostructures of graphene, hexagonal boronnitride, and alpha-RuCl3shows potential variations on a sub 10 nmlength scale. First-principles calculations reveal that the charge-doping of graphene decays sharply over just nanometers from theedge of the alpha-RuCl3flake
引用
收藏
页码:4124 / 4130
页数:7
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