Electrochemiluminescence of Water-Soluble Carbon Nanocrystals Released Electrochemically from Graphite

被引：816
作者：
Zheng, Liyan
Chi, Yuwu [1 ]
Dong, Yongqing
Lin, Jianpeng
Wang, Binbin
机构：
[1] Fuzhou Univ, Minist Educ, Key Lab Anal & Detect Food Safety, Fuzhou 350002, Peoples R China
来源：
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2009年 / 131卷 / 13期
基金：
中国国家自然科学基金;
关键词：
C-REACTIVE PROTEIN; ELECTROGENERATED CHEMILUMINESCENCE; QUANTUM DOTS; FLUORESCENT NANODIAMONDS; HIGH AMPLIFICATION; LOW CYTOTOXICITY; NANOPARTICLES; NANOTUBES; MICROSPHERES; LUMINESCENCE;
D O I：
10.1021/ja809073f
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Water-soluble carbon nanocrystals (CNCs) with electrochemiluminescence (ECL) activity were released into aqueous solution from a graphite rod by applying a scanning potential. ECL emission of CNCs observed during their preparation probably provides a useful method for monitoring and screening nanocrystal preparation. The ECL behavior and its mechanism in CNCs have been studied in detail for the first time. The results suggest promising applications of CNCs in the development of new types of biosensors and display devices in the future on the basis of their strong and stable ECL emission, good stability, low cytotoxicity, excellent water solubility, easy labeling, and environmental friendliness.
引用
收藏
页码：4564 / +
页数：3
相关论文
共 27 条
[1]   Electrochemistry and electrogenerated chemiluminescence of CdTe nanoparticles [J].
Bae, Y ;
Myung, N ;
Bard, AJ .
NANO LETTERS, 2004, 4 (06) :1153-1161
[2]   Electrochemistry and electrogenerated chemiluminescence of semiconductor nanocrystals in solutions and in films [J].
Bard, AJ ;
Ding, ZF ;
Myung, N .
SEMICONDUCTOR NANOCRYSTALS AND SILICATE NAOPARTICLES, 2005, 118 :1-57
[3]   Isolation and characterization of fluorescent nanoparticles from pristine and oxidized electric arc-produced single-walled carbon nanotubes [J].
Bottini, M ;
Balasubramanian, C ;
Dawson, MI ;
Bergamaschi, A ;
Bellucci, S ;
Mustelin, T .
JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (02) :831-836
[4]   Photoluminescent carbogenic dots [J].
Bourlinos, Athanasios B. ;
Stassinopoulos, Andreas ;
Anglos, Demetrios ;
Zboril, Radek ;
Georgakilas, Vasilios ;
Giannelis, Emmanuel P. .
CHEMISTRY OF MATERIALS, 2008, 20 (14) :4539-4541
[5]   Surface functionalized carbogenic quantum dots [J].
Bourlinos, Athanasios B. ;
Stassinopoulos, Andreas ;
Anglos, Demetrios ;
Zboril, Radek ;
Karakassides, Michael ;
Giannelis, Emmanuel P. .
SMALL, 2008, 4 (04) :455-458
[6]   Carbon dots for multiphoton bioimaging [J].
Cao, Li ;
Wang, Xin ;
Meziani, Mohammed J. ;
Lu, Fushen ;
Wang, Haifang ;
Luo, Pengju G. ;
Lin, Yi ;
Harruff, Barbara A. ;
Veca, L. Monica ;
Murray, Davoy ;
Xie, Su-Yuan ;
Sun, Ya-Ping .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (37) :11318-+
[7]  
Derfus AM, 2004, NANO LETT, V4, P11, DOI 10.1021/nl0347334
[8]   Electrochemistry and electrogenerated chemiluminescence from silicon nanocrystal quantum dots [J].
Ding, ZF ;
Quinn, BM ;
Haram, SK ;
Pell, LE ;
Korgel, BA ;
Bard, AJ .
SCIENCE, 2002, 296 (5571) :1293-1297
[9]   Characterization and application of single fluorescent nanodiamonds as cellular biomarkers [J].
Fu, Chi-Cheng ;
Lee, Hsu-Yang ;
Chen, Kowa ;
Lim, Tsong-Shin ;
Wu, Hsiao-Yun ;
Lin, Po-Keng ;
Wei, Pei-Kuen ;
Tsao, Pei-Hsi ;
Chang, Huan-Cheng ;
Fann, Wunshain .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2007, 104 (03) :727-732
[10]   Bucky light bulbs:: White light electroluminescence from a fluorescent C60 adduct-single layer organic LED [J].
Hutchison, K ;
Gao, J ;
Schick, G ;
Rubin, Y ;
Wudl, F .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1999, 121 (23) :5611-5612
123