Rotational coherence in gaseous molecules observed by the femtosecond Raman-induced polarization spectroscopy

被引:4
作者
Kohmoto, T [1 ]
Isoda, K
Fukuda, Y
Kunitomo, M
机构
[1] Kobe Univ, Fac Sci, Dept Phys, Kobe, Hyogo 6578501, Japan
[2] Kobe Univ, Grad Sch Sci & Technol, Kobe, Hyogo 6578501, Japan
关键词
ultrafast coherent beats; quantum beats; gaseous molecules; rotational coherence;
D O I
10.1016/S0022-2313(99)00484-6
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Femtosecond coherence-burst signals due to the rotational coherences in the ground vibronic state of gaseous molecules, air, nitrogen, and oxygen, were observed by using the Raman-induced polarization spectroscopy. The frequencies of the induced coherences between the relational levels are obtained from the Fourier spectrum of the coherence-burst signal. Calculations using a theory of coherent beats due to the Raman-induced rotational coherence reproduced well the observed signal and spectrum. (C) 2000 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:948 / 950
页数:3
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