Synthesis of novel nanomaterials and their application in efficient removal of radionuclides

被引:305
作者
Wang, Xiangxue [1 ]
Chen, Long [2 ]
Wang, Lin [3 ,4 ]
Fan, Qiaohui [5 ]
Pan, Duoqiang [6 ]
Li, Jiaxing [7 ]
Chi, Fangting [8 ]
Xie, Yi [7 ]
Yu, Shujun [1 ]
Xiao, Chengliang [2 ]
Luo, Feng [9 ]
Wang, Jun [10 ]
Wang, Xiaolin [11 ]
Chen, Changlun [7 ]
Wu, Wangsuo [6 ]
Shi, Weiqun [3 ,4 ]
Wang, Shuao [2 ]
Wang, Xiangke [1 ]
机构
[1] North China Elect Power Univ, Coll Environm Sci & Engn, Key Lab Resources & Environm Syst Optimizat, Minist Educ, Beijing 102206, Peoples R China
[2] Soochow Univ, State Key Lab Radiat Med & Protect, Sch Radiat Med & Protect, Collaborat Innovat Ctr Radiol Med,Jiangsu Higher, Suzhou 215123, Peoples R China
[3] Chinese Acad Sci, Inst High Energy Phys, Lab Nucl Energy Chem, Beijing 100049, Peoples R China
[4] Chinese Acad Sci, Inst High Energy Phys, Key Lab Biomed Effects Nanomat & Nanosafety, Beijing 100049, Peoples R China
[5] Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, Key Lab Petr Resources, Lanzhou 730000, Gansu, Peoples R China
[6] Lanzhou Univ, Sch Nucl Sci & Technol, Radiochem Lab, Lanzhou 730000, Gansu, Peoples R China
[7] Chinese Acad Sci, Inst Plasma Phys, CAS Key Lab Photovolta & Energy Conservat Mat, Hefei 230031, Anhui, Peoples R China
[8] Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Sichuan, Peoples R China
[9] East China Univ Technol, State Key Lab Nucl Resources & Environm, Sch Biol Chem & Mat Sci, Fuzhou 344000, Fujian, Peoples R China
[10] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Heilongjiang, Peoples R China
[11] China Acad Engn Phys, Mianyang 621900, Sichuan, Peoples R China
基金
中国国家自然科学基金;
关键词
nanomaterials; radionuclides; removal; preconcentration; interaction mechanism; ZERO-VALENT IRON; METAL-ORGANIC FRAMEWORK; 2-DIMENSIONAL TITANIUM CARBIDE; GRAPHENE OXIDE NANOSHEETS; TRANSFER RADICAL POLYMERIZATION; WALLED CARBON NANOTUBES; LAYERED DOUBLE HYDROXIDES; ABSORPTION FINE-STRUCTURE; URANIUM ADSORBENT FIBERS; NITRIC-ACID SOLUTIONS;
D O I
10.1007/s11426-019-9492-4
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
With the development of nuclear energy, large amounts of radionuclides are inevitably released into the natural environment. It is necessary to eliminate radionuclides from wastewater for the protection of environment. Nanomaterials have been considered as the potential candidates for the effective and selective removal of radionuclides from aqueous solutions under complicated conditions because of their high specific surface area, large amounts of binding sites, abundant functional groups, pore-size controllable and easily surface modification. This review mainly summarized the recent studies for the synthesis, fabrication and surface modification of novel nanomaterials and their applications in the efficient elimination and solidification of radionuclides, and discussed the interaction mechanisms from batch experiments, spectroscopy analysis and theoretical calculations. The sorption capacities with other materials, advantages and disadvantages of different nanomaterials are compared, and at last the perspective of the novel nanomaterials is summarized.
引用
收藏
页码:933 / 967
页数:35
相关论文
共 320 条
[61]   Efficient Capture of Perrhenate and Pertechnetate by a Mesoporous Zr Metal-Organic Framework and Examination of Anion Binding Motifs [J].
Drout, Riki J. ;
Otake, Kenichi ;
Howarth, Ashlee J. ;
Islamoglu, Timur ;
Zhu, Lin ;
Xiao, Chengliang ;
Wang, Shuao ;
Farha, Omar K. .
CHEMISTRY OF MATERIALS, 2018, 30 (04) :1277-1284
[62]   Experimental Measurements and Surface Complexation Modeling of U(VI) Adsorption onto Multilayered Graphene Oxide: The Importance of Adsorbate-Adsorbent Ratios [J].
Duster, Thomas A. ;
Szymanowski, Jennifer E. S. ;
Fein, Jeremy B. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2017, 51 (15) :8510-8518
[63]   Clay-supported nanoscale zero-valent iron composite materials for the remediation of contaminated aqueous solutions: A review [J].
Ezzatahmadi, Naeim ;
Ayoko, Godwin A. ;
Millar, Graeme J. ;
Speight, Robert ;
Yan, Cheng ;
Li, Jihong ;
Li, Shizhong ;
Zhu, Jianxi ;
Xi, Yunfei .
CHEMICAL ENGINEERING JOURNAL, 2017, 312 :336-350
[64]   Capture of iodine in highly stable metal-organic frameworks: a systematic study [J].
Falaise, Clement ;
Volkringer, Christophe ;
Facqueur, Jacques ;
Bousquet, Till ;
Gasnot, Laurent ;
Loiseau, Thierry .
CHEMICAL COMMUNICATIONS, 2013, 49 (87) :10320-10322
[65]   Alkalization Intercalation of MXene for Electrochemical Detection of Uranyl Ion [J].
Fan Mao ;
Wang Lin ;
Pei Cheng-Xin ;
Shi Wei-Qun .
JOURNAL OF INORGANIC MATERIALS, 2019, 34 (01) :85-90
[66]   Uranium (VI) sorption by multiwalled carbon nanotubes from aqueous solution [J].
Fasfous, Ismail I. ;
Dawoud, Jamal N. .
APPLIED SURFACE SCIENCE, 2012, 259 :433-440
[67]   A New Paradigm for Anion Trapping in High Capacity and Selectivity: Crystal-to-Crystal Transformation of Cationic Materials [J].
Fei, Honghan ;
Bresler, Marc R. ;
Oliver, Scott R. J. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (29) :11110-11113
[68]   Chelating polymer modified P84 nanofiltration (NF) hollow fiber membranes for high efficient heavy metal removal [J].
Gao, Jie ;
Sun, Shi-Peng ;
Zhu, Wen-Ping ;
Chung, Tai-Shung .
WATER RESEARCH, 2014, 63 :252-261
[69]   Recent advances about metal-organic frameworks in the removal of pollutants from wastewater [J].
Gao, Qiang ;
Xu, Jian ;
Bu, Xian-He .
COORDINATION CHEMISTRY REVIEWS, 2019, 378 :17-31
[70]  
Gao W, 2009, NAT CHEM, V1, P403, DOI [10.1038/NCHEM.281, 10.1038/nchem.281]