Electrostatic Assembly Guided Synthesis of Highly Luminescent Carbon-Nanodots@BaSO4 Hybrid Phosphors with Improved Stability

被引:121
作者
Zhou, Ding [1 ]
Zhai, Yuechen [1 ]
Qu, Songnan [1 ]
Li, Di [1 ]
Jing, Pengtao [1 ]
Ji, Wenyu [1 ]
Shen, Dezhen [1 ]
Rogach, Andrey L. [2 ,3 ]
机构
[1] Chinese Acad Sci, Changchun Inst Opt Fine Mech & Phys, State Key Lab Luminescence & Applicat, Changchun 130033, Peoples R China
[2] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China
[3] City Univ Hong Kong, Ctr Funct Photon, Kowloon, Hong Kong, Peoples R China
基金
中国国家自然科学基金;
关键词
GRAPHENE QUANTUM DOTS; LIGHT-EMITTING-DIODES; CARBON DOTS; PHOTOLUMINESCENCE; NANODOTS; FLUORESCENT; EMISSION; NANOPARTICLES; NANOCRYSTALS; THICKNESS;
D O I
10.1002/smll.201602055
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Carbon nanodots (CNDs)@BaSO4 hybrid phosphors are fabricated in an easy and low-cost process by sequentially assembling Ba2+ and SO42- ions onto the surface of carbon nanodots through electrostatic attraction. CNDs act as the nucleus to attract these reactive ions and provide the luminescent centers in the hybrid phosphors. This strategy is versatile for a variety of negatively charged CNDs with different emission colors. The advantage of the resultant hybrid phosphors is that their luminescence exhibits excellent thermal and photostability, as well as remarkable resistance to strong acid/ alkali and common organic solvents. These merits allow for the fabrication of CNDs-based light-emitting diodes using the CNDs@BaSO4 hybrid phosphors as a color conversion layer.
引用
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页数:10
相关论文
共 52 条
[1]   Luminescent Carbon Nanodots: Emergent Nanolights [J].
Baker, Sheila N. ;
Baker, Gary A. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (38) :6726-6744
[2]   Photoluminescence-Tunable Carbon Nanodots: Surface-State Energy-Gap Tuning [J].
Bao, Lei ;
Liu, Cui ;
Zhang, Zhi-Ling ;
Pang, Dai-Wen .
ADVANCED MATERIALS, 2015, 27 (10) :1663-+
[3]   Carbon Dot Loading and TiO2 Nanorod Length Dependence of Photoelectrochemical Properties in Carbon Dot/TiO2 Nanorod Array Nanocomposites [J].
Bian, Juncao ;
Huang, Chao ;
Wang, Lingyun ;
Hung, TakFu ;
Daoud, Walid A. ;
Zhang, Ruiqin .
ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (07) :4883-4890
[4]   Carbon dots for multiphoton bioimaging [J].
Cao, Li ;
Wang, Xin ;
Meziani, Mohammed J. ;
Lu, Fushen ;
Wang, Haifang ;
Luo, Pengju G. ;
Lin, Yi ;
Harruff, Barbara A. ;
Veca, L. Monica ;
Murray, Davoy ;
Xie, Su-Yuan ;
Sun, Ya-Ping .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (37) :11318-+
[5]   Photoluminescent organosilane-functionalized carbon dots as temperature probes [J].
Chen, Po-Cheng ;
Chen, Ya-Na ;
Hsu, Pin-Che ;
Shih, Chung-Chien ;
Chang, Huan-Tsung .
CHEMICAL COMMUNICATIONS, 2013, 49 (16) :1639-1641
[6]   A Self-Quenching-Resistant Carbon-Dot Powder with Tunable Solid-State Fluorescence and Construction of Dual-Fluorescence Morphologies for White Light-Emission [J].
Chen, Yonghao ;
Zheng, Mingtao ;
Xiao, Yong ;
Dong, Hanwu ;
Zhang, Haoran ;
Zhuang, Jianle ;
Hu, Hang ;
Lei, Bingfu ;
Liu, Yingliang .
ADVANCED MATERIALS, 2016, 28 (02) :312-318
[7]  
Choi H, 2013, NAT PHOTONICS, V7, P732, DOI [10.1038/nphoton.2013.181, 10.1038/NPHOTON.2013.181]
[8]   Semiconductor-Nanocrystals-Based White Light-Emitting Diodes [J].
Dai, Quanqin ;
Duty, Chad E. ;
Hu, Michael Z. .
SMALL, 2010, 6 (15) :1577-1588
[9]   Functional Surface Engineering of C-Dots for Fluorescent Biosensing and in Vivo Bioimaging [J].
Ding, Changqin ;
Zhu, Anwei ;
Tian, Yang .
ACCOUNTS OF CHEMICAL RESEARCH, 2014, 47 (01) :20-30
[10]   Full-Color Light-Emitting Carbon Dots with a Surface-State-Controlled Luminescence Mechanism [J].
Ding, Hui ;
Yu, Shang-Bo ;
Wei, Ji-Shi ;
Xiong, Huan-Ming .
ACS NANO, 2016, 10 (01) :484-491