Imaging density disturbances in water with a 41.3-attosecond time resolution

被引:57
作者
Abbamonte, P
Finkelstein, KD
Collins, MD
Gruner, SM
机构
[1] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA
[2] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.92.237401
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We show that the momentum flexibility of inelastic x-ray scattering may be exploited to invert its loss function, allowing real time imaging of density disturbances in a medium. We show the disturbance arising from a point source in liquid water, with a resolution of 41.3 attoseconds (4.13x10(-17) s) and 1.27 Angstrom (1.27x10(-8) cm). This result is used to determine the structure of the electron cloud around a photoexcited chromophore in solution, as well as the wake generated in water by a 9 MeV gold ion. We draw an analogy with pump-probe techniques and suggest that energy-loss scattering may be applied more generally to the study of attosecond phenomena.
引用
收藏
页码:237401 / 1
页数:4
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