Single layer two-dimensional O-g-C3N4: An efficient photocatalyst for improved molecular oxygen activation ability

被引:17
作者
Song, Yanhua [1 ]
She, Xiaojie [2 ]
Yi, Jianjian [2 ]
Mo, Zhao [2 ]
Liu, Liang [2 ]
Xu, Hui [2 ]
Li, Huaming [2 ]
机构
[1] Jiangsu Univ Sci & Technol, Sch Environm & Chem Engn, Zhenjiang 212003, Peoples R China
[2] Jiangsu Univ, Inst Energy Res, Zhenjiang 212013, Peoples R China
来源
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE | 2017年 / 214卷 / 05期
关键词
2D O-g-C3N4; 4-chlorophenol; organic dye; photocatalytic degradation; GRAPHITIC CARBON NITRIDE; VISIBLE-LIGHT; HYDROGEN EVOLUTION; H-2; EVOLUTION; DOPED TIO2; Z-SCHEME; G-C3N4; PERFORMANCE; PHOTODEGRADATION; PHOTOCHEMISTRY;
D O I
10.1002/pssa.201600704
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Although ultrathin two-dimensional (2D) nanomaterials have aroused great attention, the preparation methods are still difficult to meet the requirements. Herein, two-dimensional oxygen-modified single layer g-C3N4 (2D O-g-C3N4) has been prepared and used as photocatalyst for degradation of environmental pollutants. The as-prepared 2D O-g-C3N4 exhibited excellent photocatalytic activity for degradation of the organic dyes and 4-chlorophenol (4-CP). Through the DMPO spin-trapped ESR spectroscopy analysis, the photocatalytic mechanism was researched in detail. (C) 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
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页数:7
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