A TiO2 Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue

被引:28
|
作者
Zhang, Jian [1 ]
Yuan, Wei [1 ]
Xia, Tian [1 ]
Ao, Chenghong [1 ]
Zhao, Jiangqi [1 ]
Huang, Bingxue [1 ]
Wang, Qunhao [1 ]
Zhang, Wei [1 ,2 ]
Lu, Canhui [1 ,2 ]
机构
[1] Sichuan Univ, Polymer Res Inst, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China
[2] Sichuan Univ, Adv Polymer Mat Res Ctr, Shishi 362700, Peoples R China
基金
中国国家自然科学基金;
关键词
cellulose; carbon aerogel; titanium dioxide; photo-catalytic degradation; methylene blue;
D O I
10.3390/nano11010239
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Carbon aerogels (CA) derived from bamboo cellulose fibers were coupled with TiO2 to form CA/TiO2 hybrids, which exhibited extraordinary performance on the photo-catalytic degradation of methylene blue (MB). The structure and morphology of CA/TiO2 were characterized by field emission scanning electron microscopy, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and Raman spectrum. The CA displayed a highly porous and interconnected three-dimensional framework structure, while introducing the catalytic active sites of TiO2 onto the aerogel scaffold could remarkably enhance its photo-catalytic activity. The adsorption and photo-catalytic degradation of MB by the CA/TiO2 hybrid were investigated. The maximum adsorption capacity of CA/TiO2 for MB was 18.5 mg/g, which outperformed many similar materials reported in the literature. In addition, compared with other photo-catalysts, the present CA/TiO2 demonstrated superior photo-catalytic performance. Almost 85% of MB in 50 mL solution with a MB concentration of 10 mg/L could be effectively degraded by 15 mg CA/TiO2 in 300 min.
引用
收藏
页码:1 / 12
页数:12
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