Investigating fouling at the pore-scale using a microfluidic membrane mimic filtration system

被引:27
作者
Debnath, Nandini [1 ]
Kumar, Aloke [2 ]
Thundat, Thomas [3 ,4 ]
Sadrzadeh, Mohtada [1 ]
机构
[1] Univ Alberta, Dept Mech Engn, Adv Water Res Lab, 10-367 Donadeo Innovat Ctr Engn, Edmonton, AB T6G 1H9, Canada
[2] Indian Inst Sci, Dept Mech Engn, Bangalore, Karnataka, India
[3] Univ Alberta, Dept Chem & Mat Engn, Edmonton, AB T6G 2G8, Canada
[4] Univ Buffalo, Sch Engn & Appl Sci, Dept Chem & Biol Engn, Buffalo, NY 14260 USA
基金
加拿大自然科学与工程研究理事会;
关键词
WASTE-WATER TREATMENT; COLLOIDAL PARTICLES; FLOW; MODEL; FLUX; ULTRAFILTRATION; DEPOSITION; STREAMERS; MICROFILTRATION; REJECTION;
D O I
10.1038/s41598-019-47096-6
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The work investigates fouling in a microfluidic membrane mimic (MMM) filtration system for foulants such as polystyrene particles and large polymeric molecules. Our MMM device consists of a staggered arrangement of pillars which enables real-time visualization and analysis of pore-scale phenomena. Different fouling scenarios are investigated by conducting constant-pressure experiments. Fouling experiments are performed with three different types of foulants: polystyrene particle solution (colloidal fouling), polyacrylamide polymer solution (organic fouling) and a mixture of these two solutions (combined fouling). Four major categories of microscopic fouling are observed: cake filtration (upstream), pore blocking (inside the pores), colloidal aggregation (downstream) and colloidal streamer fouling (downstream). Our microfluidic experiments show that downstream colloidal aggregation and streamer fouling have a significant effect on overall membrane fouling which were not studied before.
引用
收藏
页数:10
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