Efficient conversion of NO with CeO2/TiO2 using non-thermal plasma

被引:0
|
作者
Adwek, George [1 ]
Shen, Boxiong [1 ]
Yang, Jiancheng [1 ]
Siagi, Zachary [2 ]
Wang, Jianqiao [1 ]
Cicilia, Kemunto M. [1 ]
Arowo, Moses [2 ]
Julius, Gane [3 ]
Kang, Dongrui [1 ]
机构
[1] Hebei Univ Technol, Sch Energy & Environm Engn, Tianjin, Peoples R China
[2] Moi Univ, Sch Engn, Eldoret, Kenya
[3] Univ Leeds, Energy Res Inst, Leeds LS2 9JT, W Yorkshire, England
基金
美国国家科学基金会;
关键词
SELECTIVE CATALYTIC-REDUCTION; FLUE-GAS; REMOVAL; CORONA; DISCHARGE; TEMPERATURE;
D O I
10.1088/1755-1315/227/6/062007
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Alternating current (AC) dielectric barrier discharge induced non-thermal plasma (NTP) has been used to experimentally investigate conversion of Nitrogen Oxide (NO) over CeO2/TiO2 catalyst. The role of heterogeneous catalyst (TiO2/CeO2) has also been investigated, NO conversion has been examined in terms of various operating parameters including temperature, voltage, flue gas flow rate, specific energy density, water vapour content and oxygen content. The conversion mechanism of NO was distinctly discussed. To understand the effects of NTP on CeO2/TiO2 catalyst properties and the influence of CeO2/TiO2 catalyst on NTP, SEM, BET, XRD, TPR were carried out. SEM reveals that increase in temperature during NTP catalytic reactions affect the morphology of the catalyst hence decreasing NO oxidation efficiency, the results also show that surface area and pore properties of the catalyst plays a significant role in plasma catalytic reaction. The maximum NO oxidation conversion efficiency attained was 93% at SED of 91JL(-1)
引用
收藏
页数:12
相关论文
共 50 条
  • [1] Removal of toluene by non-thermal plasma combined with photocatalyst TiO2
    School of Environmental Science and Engineering, South China University of Technology, Guangzhou 510006, China
    Huanan Ligong Daxue Xuebao, 2008, 11 (27-33):
  • [2] Efficient degradation of chlorobenzene in a non-thermal plasma catalytic reactor supported on CeO2/HZSM-5 catalysts
    Jiang, Liying
    Nie, Guofeng
    Zhu, Runye
    Wang, Jiade
    Chen, Jianmeng
    Mao, Yubo
    Cheng, Zhuowei
    Anderson, Willam A.
    JOURNAL OF ENVIRONMENTAL SCIENCES, 2017, 55 : 266 - 273
  • [3] Efficient degradation of chlorobenzene in a non-thermal plasma catalytic reactor supported on CeO2/HZSM-5 catalysts
    Liying Jiang
    Guofeng Nie
    Runye Zhu
    Jiade Wang
    Jianmeng Chen
    Yubo Mao
    Zhuowei Cheng
    Willam A.Anderson
    Journal of Environmental Sciences, 2017, 55 (05) : 266 - 273
  • [4] Efficient activation of Pd/CeO2 catalyst by non-thermal plasma for complete oxidation of indoor formaldehyde at room temperature
    Li, Kai
    Ji, Jian
    Huang, Haibao
    He, Miao
    CHEMOSPHERE, 2020, 246
  • [5] Non-Thermal Plasma Assisted Regeneration of Acetone Adsorbed TiO2 Surface
    Sivachandiran, L.
    Thevenet, F.
    Rousseau, A.
    PLASMA CHEMISTRY AND PLASMA PROCESSING, 2013, 33 (05) : 855 - 871
  • [6] Non-Thermal Plasma Assisted Regeneration of Acetone Adsorbed TiO2 Surface
    L. Sivachandiran
    F. Thevenet
    A. Rousseau
    Plasma Chemistry and Plasma Processing, 2013, 33 : 855 - 871
  • [7] Air non-thermal plasma treatment of Irgarol 1051 deposited on TiO2
    Giardina, Agata
    Tampieri, Francesco
    Marotta, Ester
    Paradisi, Cristina
    CHEMOSPHERE, 2018, 210 : 653 - 661
  • [8] Efficient Photodegradation of Gasoline Additives MTBE and ETBE with TiO2 and CeO2
    Hejda, S.
    Kluson, P.
    Janos, P.
    Zlamal, M.
    PROCEEDINGS OF THE 6TH EUROPEAN MEETING ON SOLAR CHEMISTRY & PHOTOCATALYSIS: ENVIRONMENTAL APPLICATIONS, 2010, : 324 - 324
  • [9] CeO2/CuO/TiO2 heterojunction photocatalysts for conversion of CO2 to ethanol
    Seeharaj, Panpailin
    Vittayakorn, Naratip
    Morris, John
    Kim-Lohsoontorn, Pattaraporn
    NANOTECHNOLOGY, 2021, 32 (37)
  • [10] MnOx/TiO2 Catalysts for VOCs Abatement by Coupling Non-thermal Plasma and Photocatalysis
    Aouadi, I.
    Tatibouet, J. -M.
    Bergaoui, L.
    PLASMA CHEMISTRY AND PLASMA PROCESSING, 2016, 36 (06) : 1485 - 1499