Differing Mechanisms of New Particle Formation at Two Arctic Sites

被引：103

作者：

Beck, Lisa J. ^{[1
]}

Sarnela, Nina ^{[1
]}

Junninen, Heikki ^{[1
,2
]}

Hoppe, Clara J. M. ^{[3
]}

Garmash, Olga ^{[1
]}

Bianchi, Federico ^{[1
]}

Riva, Matthieu ^{[1
,18
]}

Rose, Clemence ^{[1
,19
]}

Perakyla, Otso ^{[1
]}

Wimmer, Daniela ^{[1
]}

Kausiala, Oskari ^{[1
]}

Jokinen, Tuija ^{[1
]}

Ahonen, Lauri ^{[1
]}

Mikkila, Jyri ^{[1
]}

Hakala, Jani ^{[1
]}

He, Xu-Cheng ^{[1
]}

Kontkanen, Jenni ^{[1
]}

Wolf, Klara K. E. ^{[6
]}

Cappelletti, David ^{[4
]}

Mazzola, Mauro ^{[5
]}

Traversi, Rita ^{[5
,6
]}

Petroselli, Chiara ^{[4
]}

Viola, Angelo P. ^{[7
]}

Vitale, Vito ^{[5
]}

Lange, Robert ^{[8
]}

Massling, Andreas ^{[8
]}

Nojgaard, Jakob K. ^{[8
]}

Krejci, Radovan ^{[9
,10
]}

Karlsson, Linn ^{[9
,10
]}

Zieger, Paul ^{[9
,10
]}

Jang, Sehyun ^{[11
]}

Lee, Kitack ^{[11
]}

Vakkari, Ville ^{[12
,13
]}

Lampilahti, Janne ^{[1
]}

Thakur, Roseline C. ^{[1
]}

Leino, Katri ^{[1
]}

Kangasluoma, Juha ^{[1
,14
]}

Duplissy, Ella-Maria ^{[1
]}

Siivola, Erkki ^{[1
]}

Marbouti, Marjan ^{[1
]}

Tham, Yee Jun ^{[1
]}

Saiz-Lopez, Alfonso ^{[15
]}

Petaja, Tuukka ^{[1
]}

Ehn, Mikael ^{[1
]}

Worsnop, Douglas R. ^{[1
,16
]}

Skov, Henrik ^{[8
]}

Kulmala, Markku ^{[1
,17
]}

Kerminen, Veli-Matti ^{[1
]}

Sipila, Mikko ^{[1
]}

机构：

[1] Univ Helsinki, Fac Sci, Inst Atmospher & Earth Syst Res Phys, Helsinki, Finland

[2] Univ Tartu, Inst Phys, Lab Environm Phys, Tartu, Estonia

[3] Helmholtz Zentrum Polar & Meeresforsch, Alfred Wegener Inst, Bremerhaven, Germany

[4] Univ Perugia, Dept Chem Biol & Biotechnol, Perugia, Italy

[5] CNR, Inst Polar Sci, Bologna, Italy

[6] Univ Florence, Dept Chem, Florence, Italy

[7] CNR, Inst Polar Sci, Montelibretti, Italy

[8] Aarhus Univ, IClimate, Dept Environm Sci, Roskilde, Denmark

[9] Stockholm Univ, Dept Environm Sci, Stockholm, Sweden

[10] Stockholm Univ, Bolin Ctr Climate Res, Stockholm, Sweden

[11] Pohang Univ Sci & Technol, Div Environm Sci & Engn, Pohang, South Korea

[12] Finnish Meteorol Inst, Helsinki, Finland

[13] North West Univ, Atmospher Chem Res Grp, Potchefstroom, South Africa

[14] Beijing Univ Chem Technol, Aerosol & Haze Lab, Beijing Adv Innovat Ctr Soft Matter Sci & Engn, Beijing, Peoples R China

[15] CSIC, Inst Phys Chem Rocasolano, Dept Atmospher Chem & Climate, Madrid, Spain

[16] Aerodyne Res Inc, Billerica, MA USA

[17] Nanjing Univ, Joint Int Res Lab Atmospher & Earth Syst Sci, Nanjing, Peoples R China

[18] Univ Claude Bernard Lyon 1, Univ Lyon, Villeurbanne, France

[19] Lab Meteorol Phys, Aubiere, France

来源：

GEOPHYSICAL RESEARCH LETTERS | 2021年 / 48卷 / 04期

基金：

芬兰科学院; 欧洲研究理事会; 瑞典研究理事会; 奥地利科学基金会; 新加坡国家研究基金会;

关键词：

Arctic atmosphere; low‐ volatility vapors; new particle formation; FORMATION EVENTS; SULFURIC-ACID; ATMOSPHERIC PARTICLES; OCEANIC PHYTOPLANKTON; METHANESULFONIC-ACID; SIZE DISTRIBUTIONS; MASS-SPECTROMETER; AEROSOL FORMATION; RESEARCH STATION; NEUTRAL CLUSTER;

D O I：

10.1029/2020GL091334

中图分类号：

P [天文学、地球科学];

学科分类号：

07 ;

摘要：

New particle formation in the Arctic atmosphere is an important source of aerosol particles. Understanding the processes of Arctic secondary aerosol formation is crucial due to their significant impact on cloud properties and therefore Arctic amplification. We observed the molecular formation of new particles from low-volatility vapors at two Arctic sites with differing surroundings. In Svalbard, sulfuric acid (SA) and methane sulfonic acid (MSA) contribute to the formation of secondary aerosol and to some extent to cloud condensation nuclei (CCN). This occurs via ion-induced nucleation of SA and NH3 and subsequent growth by mainly SA and MSA condensation during springtime and highly oxygenated organic molecules during summertime. By contrast, in an ice-covered region around Villum, we observed new particle formation driven by iodic acid but its concentration was insufficient to grow nucleated particles to CCN sizes. Our results provide new insight about sources and precursors of Arctic secondary aerosol particles.

引用

页数：11

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