Thermal vestige of the zero-temperature jamming transition

被引:235
|
作者
Zhang, Zexin [1 ]
Xu, Ning [1 ,2 ]
Chen, Daniel T. N. [1 ]
Yunker, Peter [1 ]
Alsayed, Ahmed M. [1 ]
Aptowicz, Kevin B. [3 ]
Habdas, Piotr [4 ]
Liu, Andrea J. [1 ]
Nagel, Sidney R. [2 ]
Yodh, Arjun G. [1 ]
机构
[1] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA
[2] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA
[3] W Chester Univ, Dept Phys, W Chester, PA 19383 USA
[4] St Josephs Univ, Dept Phys, Philadelphia, PA 19131 USA
基金
美国国家科学基金会;
关键词
COLLOIDAL CRYSTALS; VIDEO MICROSCOPY; GLASS-TRANSITION; SUSPENSIONS; RELAXATION; PARTICLES; DYNAMICS; MIXTURE;
D O I
10.1038/nature07998
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
When the packing fraction is increased sufficiently, loose particulates jam to form a rigid solid in which the constituents are no longer free to move. In typical granular materials and foams, the thermal energy is too small to produce structural rearrangements. In this zero-temperature (T = 0) limit, multiple diverging(1-8) and vanishing(2,9,10) length scales characterize the approach to a sharp jamming transition. However, because thermal motion becomes relevant when the particles are small enough, it is imperative to understand how these length scales evolve as the temperature is increased. Here we used both colloidal experiments and computer simulations to progress beyond the zero-temperature limit to track one of the key parameters-the overlap distance between neighbouring particles-which vanishes at the T = 0 jamming transition. We find that this structural feature retains a vestige of its T = 0 behaviour and evolves in an unusual manner, which has masked its appearance until now. It is evident as a function of packing fraction at fixed temperature, but not as a function of temperature at fixed packing fraction or pressure. Our results conclusively demonstrate that length scales associated with the T = 0 jamming transition persist in thermal systems, not only in simulations but also in laboratory experiments.
引用
收藏
页码:230 / 233
页数:4
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