Strong dependence of dielectric properties on electrical boundary conditions and interfaces in ferroelectric superlattices

被引:19
作者
Misirlioglu, I. B. [1 ]
Kesim, M. T. [2 ,3 ]
Alpay, S. P. [2 ,3 ,4 ]
机构
[1] Sabanci Univ, Fac Engn & Nat Sci, TR-34956 Istanbul, Turkey
[2] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA
[3] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA
[4] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA
关键词
THIN-FILMS; PHASE-TRANSITIONS; BATIO3/SRTIO3; SUPERLATTICES; MULTILAYERS; GROWTH;
D O I
10.1063/1.4862408
中图分类号
O59 [应用物理学];
学科分类号
摘要
A computational study based on Landau-Ginzburg-Devonshire theory is carried out to understand the role of interfaces on the dielectric response of ferroelectric superlattices. Using heteroepitaxial (001) PbZr0.3Ti0.7O3/(001)SrTiO3 heterostructures on (001)SrTiO3 as an example, we show that electrostatic boundary conditions have a pronounced effect on the dielectric response far below the ferroelectric phase transition temperature. For a fixed total multilayer thickness, the average dielectric response can be improved significantly for superlattices with a small layer periodicity. This is due to the large total internal electric fields at the interlayer interfaces which originate from the polarization mismatch between layers. (C) 2014 AIP Publishing LLC.
引用
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页数:5
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共 37 条
[21]   Phase transitions and strain-induced ferroelectricity in SrTiO3 epitaxial thin films [J].
Pertsev, NA ;
Tagantsev, AK ;
Setter, N .
PHYSICAL REVIEW B, 2000, 61 (02) :R825-R829
[22]   Phase diagrams and physical properties of single-domain epitaxial Pb(Zr1-xTix)O3 thin films -: art. no. 054107 [J].
Pertsev, NA ;
Kukhar, VG ;
Kohlstedt, H ;
Waser, R .
PHYSICAL REVIEW B, 2003, 67 (05)
[23]   Dielectric anomaly due to electrostatic coupling in ferroelectric-paraelectric bilayers and multilayers [J].
Roytburd, AL ;
Zhong, S ;
Alpay, SP .
APPLIED PHYSICS LETTERS, 2005, 87 (09)
[24]   Strain tuning of ferroelectric thin films [J].
Schlom, Darrell G. ;
Chen, Long-Qing ;
Eom, Chang-Beom ;
Rabe, Karin M. ;
Streiffer, Stephen K. ;
Triscone, Jean-Marc .
ANNUAL REVIEW OF MATERIALS RESEARCH, 2007, 37 :589-626
[25]   PHASE-TRANSITIONS AND SOFT MODES IN FERROELECTRIC SUPERLATTICES [J].
SCHWENK, D ;
FISHMAN, F ;
SCHWABL, F .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1990, 2 (24) :5409-5431
[26]   Growth of nanoscale BaTiO3/SMO3 superlattices by molecular-beam epitaxy [J].
Soukiassian, A. ;
Tian, W. ;
Vaithyanathan, V. ;
Haeni, J. H. ;
Chen, L. Q. ;
Xi, X. X. ;
Schlom, D. G. ;
Tenne, D. A. ;
Sun, H. P. ;
Pan, X. Q. ;
Choi, K. J. ;
Eom, C. B. ;
Li, Y. L. ;
Jia, Q. X. ;
Constantin, C. ;
Feenstra, R. M. ;
Bernhagen, M. ;
Reiche, P. ;
Uecker, R. .
JOURNAL OF MATERIALS RESEARCH, 2008, 23 (05) :1417-1432
[27]   X-ray diffraction measurement of the effect of layer thickness on the ferroelectric transition in epitaxial KTaO3/KNbO3 multilayers [J].
Specht, ED ;
Christen, HM ;
Norton, DP ;
Boatner, LA .
PHYSICAL REVIEW LETTERS, 1998, 80 (19) :4317-4320
[28]   Domain-enhanced interlayer coupling in ferroelectric/paraelectric superlattices [J].
Stephanovich, VA ;
Luk'yanchuk, IA ;
Karkut, MG .
PHYSICAL REVIEW LETTERS, 2005, 94 (04)
[29]   Challenges and opportunities for multi-functional oxide thin films for voltage tunable radio frequency/microwave components [J].
Subramanyam, Guru ;
Cole, M. W. ;
Sun, Nian X. ;
Kalkur, Thottam S. ;
Sbrockey, Nick M. ;
Tompa, Gary S. ;
Guo, Xiaomei ;
Chen, Chonglin ;
Alpay, S. P. ;
Rossetti, G. A., Jr. ;
Dayal, Kaushik ;
Chen, Long-Qing ;
Schlom, Darrell G. .
JOURNAL OF APPLIED PHYSICS, 2013, 114 (19)
[30]   FORMATION OF ARTIFICIAL BATIO3/SRTIO3 SUPERLATTICES USING PULSED-LASER DEPOSITION AND THEIR DIELECTRIC-PROPERTIES [J].
TABATA, H ;
TANAKA, H ;
KAWAI, T .
APPLIED PHYSICS LETTERS, 1994, 65 (15) :1970-1972